Art PowerPoints Harris: Quantitative Chemical Analysis, Eight Edition CHAPTER 14: ELECTRODES AND POTENTIOMETRY.

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Presentation transcript:

Art PowerPoints Harris: Quantitative Chemical Analysis, Eight Edition CHAPTER 14: ELECTRODES AND POTENTIOMETRY

CHAPTER 14: Figure Reference Electrodes

CHAPTER 14: Figure 14.2

CHAPTER 14: Figure 14.3 Ag|AgCl|Cl - (xM) Reference Electrode

CHAPTER 14: Figure 14.4

CHAPTER 14: Figure 14.5 Calomel Electrode

CHAPTER 14: Figure 14.6

CHAPTER 14: Equation 14.18

CHAPTER 14: Figure 14.7 Indicator Electrode

CHAPTER 14: Equation Potentiometric Titration

CHAPTER 14: Figure 14.8 Potentiometric Titration

CHAPTER 14: Equation 14.2

CHAPTER 14: Equation 14.3

CHAPTER 14: Figure 14.9 Junction Potential

CHAPTER 14: Table 14.1

CHAPTER 14: Table 14.2

CHAPTER 14: Figure 14.10

CHAPTER 14: Equation 14.20

CHAPTER 14: Equation 14.21

CHAPTER 14: Equation 14.4

CHAPTER 14: Equation 14.22

CHAPTER 14: Equation 14.5

CHAPTER 14: Equation pH Measurement with a Glass Electrode

CHAPTER 14: Figure 14.11

CHAPTER 14: Figure 14.12

CHAPTER 14: Figure 14.13

CHAPTER 14: Unnumbered Figure 14.7

CHAPTER 14: Equation 14.6

CHAPTER 14: Figure 14.14

CHAPTER 14: Figure 14.15

CHAPTER 14: Equation 14.7

CHAPTER 14: Figure 14.16

CHAPTER 14: Table 14.3a

CHAPTER 14: Table 14.3b

Errors in pH Measurement 1.Standards 2.Junction potential 3.Junction potential drift 4.Sodium error 5.Acid error 6.Equilibration time 7.Hydration of glass 8.Temperature 9.Cleaning

CHAPTER 14: Figure Junction potential drift

CHAPTER 14: Figure Acid and sodium (alkaline) error

CHAPTER 14: Figure Not all pH electrodes are glass IrO 2 (s) + H + + e - ↔ IrOOH(s) Can measure pH in a confined area or under extreme conditions Ion-Selective Electrodes 1.Glass membranes 2.Solid-state electrodes 3.Liquid-based electrodes 4.Compound electrodes

CHAPTER 14: Equation 14.9 Selectivity coefficient The smaller the selectivity coefficient, the less the interference by X. Example: valinomycin : selective chelator of K + Response of ion-selective electrode

CHAPTER 14: Equation Using the selectivity coefficient Q: A fluoride ion-selective electrode has a selectivity coefficient of 0.1 for OH -. What will be the change in electrode potential when 1.0 x M F - at pH 5.5 is raised to pH 10.5? Solution At pH 5.5, E = constant – log(1.0 x (0.1)( )) = constant mV At pH 10.5, E = constant – log(1.0 x (0.1)( )) = constant mV Difference = -7.1 mV: quite significant!

CHAPTER 14: Equation Solid-State Electrodes

CHAPTER 14: Figure 14.21

CHAPTER 14: Table 14.5

CHAPTER 14: Figure 14.22

CHAPTER 14: Equation Liquid-Based Ion-Selective Electrodes A hydrophobic membrane is impregnated with a hydrophobic ion exchanger called an ionophore.

CHAPTER 14: Figure Breakthrough in Ion-Selective Electrode Detection Limit Using a Metal Ion Buffer

CHAPTER 14: Table 14.6

CHAPTER 14: Figure Compound Electrodes

CHAPTER 14: Equation Standard Addition with ISE S = βRT/nF

CHAPTER 14: Equation Metal Ion Buffers By changing the ratio of [MY n-4 ] and [EDTA], [M n+ ] can be determined. – metal ion concentration can be maintained constant.

CHAPTER 14: Figure Solid-State Chemical Sensors

CHAPTER 14: Figure 14.32

CHAPTER 14: Figure 14.33

CHAPTER 14: Figure 14.34

CHAPTER 14: Figure 14.35

CHAPTER 14: Figure 14.37

CHAPTER 14: Figure 14.36

Homework Problems of Chapter , 9, 11, 16, 26, 33, 35, 40, 42, 45