Urban pollution modeling

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Urban pollution modeling using synoptic and local scale meteorological data A. RUSSO (1), R.M. TRIGO (1), P. LIND (2), F. RAISCHEL (1), M. MENDES (3) (1) IDL, University of Lisbon, Lisbon, Portugal; (2) ForWind, Institute of Physics, Carl-von-Ossietzky University of Oldenburg, Germany; (3) IPMA, Rua C-Aeroporto,1749-077 Lisbon, Portugal Objectives Air pollution (AP) is a complex mixture of toxic components that might have serious impacts on human health and quality of life, especially for sensitive groups [1]. Short term forecasting models emerge as an effective approach in order to identify and predict episodes of high pollution levels. Results The most significant variables in predicting PM10 are pollutants related to road traffic emissions and meteorological variables related to atmospheric stability. The RES-7 approach presented the best results (Tables 1,2 and Fig. 4). Moreover, MLR and NN showed similar performances when evaluated by several performance criteria (Pearson Correlation (PC), skill against persistence (SSp), root mean square error (RMSE), false alarm rates (F and F50) and percent of correctness (PC and PC50). Method The selection of variables was made independently for each monitoring station through a forward stepwise regression. Linear (MLR) and non-linear (NN) neural networks (Fig. 3), which are mathematical models inspired by the biological nervous system [2], were applied in order to produce PM10 daily forecasts. MLR models were trained with the Widrow-Hoff rule and the NN models with the Levenberg-Marquardt method. A cross-validation was applied with the available period being divided and the calibration-validation procedure was completed four times independently. Two modeling approaches were tested: a) model the original PM10 concentrations (TOT); b) model the residual component after the removal of a periodic component from the original data, namely the weekly cycle (RES-7). This work main goal is to test the potential predictive capability of linear and non-linear neural network models when applied to the concentration of PM10 measured at the urban area of Lisbon (Figs. 1,2), Portugal. The interaction between meteorological variables and PM10 was studied locally between 2002 and 2006. Table 1: Average performance indicators obtained for the PM10 calibration/validation process Fig. 4 Scatter plots of MLR results versus actual observed PM10 values for all monitoring stations and for the year 2006. Fig. 1 Case study area and stations Conclusions Results show that good predictions of PM10 are possible, if the local meteorological situation described through the CWTs and complementary meteorological data is taken into account. Models achieved good predictive performance with high values of PC, SSp, PC, and a low F. Similarly to previous studies for other pollutants, our validation results show that linear models on average perform as well or better as non-linear models for PM10. Data Daily mean NO2, NO, CO, PM10 Daily maximum PM10 PM10 at 00:00 UTC Daily circulation weather type (CWT) Boundary layers heights (03:00, 09:00, 21:00 UTC) Daily maximum temperature Daily mean wind direction and intensity Daily mean humidity and radiance Table 2: PC between observed and modelled PM10 for each station for 2002-2005 and for the independent forecast year (2006). Fig. 3 Illustration of a feed-forward artificial neural network model with three layers. Input variables Xi=1,...,p can be perceived as “neurons”, ω Represent the weights associated to each neuron and b are the bias vectors which combined will produce an output within certain error limits. REFERENCES [1] Russo, A., Raischel, F., Lind, P.G., 2013. Air quality prediction using optimal neural networks with stochastic variables, Atmospheric Environment, 79, 822-830, ISSN 1352-2310, http://dx.doi.org/10.1016/j.atmosenv.2013.07.072. [2] Cobourn, W., Dolcine, L., French, M., Hubbard, M., 2000. A comparison of nonlinear regression and neural network models for ground-level ozone forecasting. Journal of the Air & Waste Management Association, 50, 1999-2009. Fig. 2 Daily PM10 at Av. Liberdade Acknowledgments The authors acknowledge the Instituto do Mar e da Atmosfera and the Agência Portuguesa do Ambiente for the meteorological and environmental data, respectively. The authors also acknowledge Deutscher Akademischer Auslandsdienst (DAAD) and Fundação para a Ciência e Tecnologia (FCT) through the bilateral cooperation DRI/DAAD/1208/2013 (FR and PGL) and FCT for support through SFRH/BPD/65427/2009 (FR), and through Ref. PEst-OE/FIS/UI0618/2011 (FR). PL thanks BMU (German Environment Ministery) under the project 41V6451.