Triple-Humped Fission Barrier and Clusterization in the Actinide Region A. Krasznahorkay Inst. of Nucl. Res. of the Hungarian Acad. of Sci. (ATOMKI) Debrecen,

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Presentation transcript:

Triple-Humped Fission Barrier and Clusterization in the Actinide Region A. Krasznahorkay Inst. of Nucl. Res. of the Hungarian Acad. of Sci. (ATOMKI) Debrecen, Hungary

Experimental results: Introduction Resonant tunneling Experimental methods Experimental results: Superdeformed (SD) bands in 240Pu Hyperdeformed (HD) bands in 234U and in 236U On the shape of the potential barriers Mass distributions for 236U and for 233Th Clustering effects Summary and conclusion

Triple humped fission barrier

Nuclear fission paths

Resonant tunneling through the fission barrier Eres  E*, ()  J,K

The best energy regions for studying the SD and HD states Howard, Möller, ADNDT 25 (1980) 218 Cwiok et al., PLB 322 (1994) 304

Cyclotron laboratory in ATOMKI, Debrecen

The split-pole magnetic spectrometer in ATOMKI

Experimental setup for studying fission (transmission) resonances in ATOMKI (Debrecen)

Low-pressure position sensitive avalanche counters

Experimental setup for studying fission resonances in Garching (Germany)

Experimental results for 240Pu

SD rotational bands in 240Pu

Previous results for 234U P.G. Goldstone et al., PRC 18 (1978) 1706 J. Blons et al., NP A477 (1988) 21 A. Krasznahorkay et al., PRL 80 (1998) 2073

Reanalized angular distributions

Comparison of the results obtained for 234U

Recent results for 234U A. Krasznahorkay et al., Phys. Lett B 461 (1999) 15

Results of the fitting

Previous results for 236U Krasznahorkay et al., PRL 80 (1998) 2073 P.G. Goldstone et al., PRC 18 (1978) 1706

Angular distribution of the 5.4 MeV band in 236U

Recent results for 236U

Fitting the fission resonances in 236U Not SD but HD bands !!!

On the depth of the third minimum Calculations with the back shifted Fermi-gas model

Determination of the height of the inner barrier Lower and higher limits  EA= 5.15 ± 0.20 MeV hA = 1.2 MeV Exp. Data from Goerlach diploma thesis, Univ. MPI Heidelberg (1978), unpublished

On the height of the fission barriers History of the 3. Minimum Möller … PLB 40 (1972) 329 Blons … PRL 41 (1978) 1282 (Howard, Möller, ADNDT 25 (1980) 218 ) Cwiok … PLB 322 (1994) 304

Nuclear molecules

Clusterization in 234U

The shape of 236U in the third minimum

Setup for TOF measurements

On the width of the mass distribution of 236U

Mass distribution measurements with a double ionization chamber C. Budtz-Jörgensen et al., NIM A258 (1987) 209

On the width of the mass distributions of 233Th Target: ThO2 0.1 mg/cm2, diameter 4 cm Neutrons from 7Li(p,n) at ATOMKI then in Karlsruhe, =1.8*106 n/cm2, one week exp.

TKE-mass distribution correlations A=100 A=132 Cold fission Compact fission

TKE-mass correlations in the decay of the HD resonance in 233Th

Summary and conclusions Fission resonances  SD and HD states Density of the HD states  depth of the 3rd minimum Appearence of the HD resonances + isomer population probability  EA The ˝Th anomaly˝ has been solved. Mass distribution from the decay of the HD states  heavy clusterization