More on Fission Products

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Presentation transcript:

More on Fission Products  and  emissions from radioactive fission products carry part of the fission energy, even after shut down. On approaching end of the chain, the decay energy decreases and half-life increases. Long-lived isotopes constitute the main hazard. Can interfere with fission process in the fuel. (poisoning). Important for research. -decay favors high energy  17 MeV compared to 6 MeV for . Only 7 MeV from -decay appears as heat. Why? Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning Not anticipated! Reactor shut down! 135Xe 106 b Time scale: Hours and days. 135Xe 106 b 149Sm 105 b Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning HW 48 Negative reactivity due to poison buildup. It is proportional to the amount of poison. Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Assume no spacial dependence. Poisoning small Initial conditions? Clean Core Startup. Shutdown (later). Assume no spacial dependence. Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning The solution is and Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning Now, we know Xe(t) Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning Shutdown. After the reactor has been operating for a “long” time. Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning The solution is > 0 ? Height of the peak depends on I() and Xe(), i.e. depends on . Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning Shutdown  Xe   negative   move control rods out  try to add positive reactivity  need to have enough reserve  costly to do that. If, the available excess reactivity can compensate for less than 30 minutes of poison buildup, can’t startup again after ~30 minutes of shutdown, because you can’t achieve criticality. Need to wait some 40 hours (in this case) for Xe to decay down. Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning Strategies If you plan to shut down for “short maintenance”, think about stepback. Examine different scenarios using this code from http://www.nuceng.ca/ You will get more experience after you finish the computational physics course. Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning Xe Oscillations (r,t) (spacial dependence)  flux  locally  Xe burnup    (reactivity)   flux further   control rods globally in  flux  elsewhere  Xe burnup     ….. Xe oscillation but limited by opposite effect due to increase (decrease) of I in the high (low) flux region. In large reactors (compared to neutron diffusion length) local flux, power and temperature could reach unacceptable values for certain materials  safety issues. Think of one sensor and one control rod  feel average flux  apparently OK  more sensors and control rods to locate and deal with local changes. Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Poisoning Permanent Poisons 149Sm has sizeable but lower cross section than 135Xe. It does not decay. Start from fresh fuel: Thus: Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Radioactive Fission Products Read section 13.7 in Krane. Look at sections 13.8 and 13.9 Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Radioactive Fission Products per watt of original operating power. T = time of operation. Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).

Radioactive Fission Products Nuclear and Radiation Physics, BAU, First Semester, 2007-2008 (Saed Dababneh).