Debye-like shielding effect on low-cloud electricity by the radioactive aerosol after Fukushima nuclear accident M. Yamauchi1, M. Takeda2, M. Makino3,

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Debye-like shielding effect on low-cloud electricity by the radioactive aerosol after Fukushima nuclear accident M. Yamauchi1, M. Takeda2, M. Makino3, and T. Owada4 (1) Swedish Institute of Space Physics (IRF), Kiruna, Sweden (2) Kyoto University, Japan (3) National Institute of Advanced Industrial Science and Technology, Tsukuba, Japan (4) Kakioka Magnetic Observatory, Japan Meteorological Agency, Ishioka, Japan R117@GI1.4 (EGU2014-3713) Monday 2014-04-28 1

Effect of ionizing radiation Instrument to measure E-field 2 Extra ionization decreases the atmospheric E-field (PG) (Kakioka PG sampling is 1 Hz. Data is calibrated and compared with backup measurement)

observed PG drop Helsinki, 1986 Tucson, 1952 Rain Rain 24 hours 2 weeks PG drops after Chernobyl Accident (Tuomi, 1988) PG drops after nuclear test (Harris, 1955) 3

Past analyses = PG under clear sky (A) 14-20 March = floating radionuclide 14 March: Dry deposition on 14 March at Kakioka, 150 km. 16-20 March: Strong re-suspension by wind. (B) - 20 April = some re-suspension & occasional plumes from FNPP-1 20-21 March: Wet deposition at Kakioka by the first substantial rain. until around 20 April : Transport from highly-contaminated to moderately-contaminated areas by daily wind. (C) afterward = minor plumes until summer from FNPP-1 4

What about rain-time PG? Example (1-h data) after before Difficulty (reason why no work for Chernobyl and nuclear tests): PG under rain-cloud is highly variable and dynamic Reliability of observation is not well established  yet worth examining whether there is statistical difference 5

Survey of 2006-2013: Percent of "negative spikes" for different rain conditions Largest difference in PG value between 2011 and the other years are during weak rain or right before/after the rain 6

Our Statistics Use 1-min value data (binned every 15 min) Examine all positive and negative peaks (no comparison to rain data to increase statistics) Remove even minor peaks (see illustration) 7 Less occurrence of -100 ~ -800 V/m (most likely minor rain) in 2011

time scale (overview) March-April May Quick decay & development for 2011 Effect ended by May May 8 Relative PG values compared to the peak during 5 min before and 5 min after.

time scale (detail) The difference is most clear for peak values of -200 ~ -400 V/m May () is already back to normal (consistent with the end of re- suspension). 9

Interpretation Extra ionization of aerosols in the lower atmosphere by the ionizing radiation except during heavy rain that washes out these aerosols.  Quicker response to the change in the cloud-origin electric field Increase of electric conductivity ~x10 near ground and x 1.5~3 at higher 10

consequence of high  There are two way of describing the response of ionized aerosols to E: Shorter "re-distribution" time of ionized aerosols to respond changes in the cloud electricity (by internal convection + cloud motion). Shorter "shielding distance" of quasi-neutral atmosphere. This extra effect to (1) keeps aerosols more dielectric rather than conductive Increase of ions results more shielding (i.e., decrease of shielding distance D). D for time scale < 5 min depends on ion density & how quickly ions moves  D   when  (conductivity) is very low Just doubling D (~1/4) makes substantial difference D ~ /ionosphere * (D)ionosphere ~ 1~10 km  agrees with observation 11

Summary 10-min averaged PG during weak rain or just before/after the rain is not as large right after the Fukushima accident as the same season of the other years This difference is due to the shorter time scale toward/from the peak during the time that ionizing radiation increased. The behavior is consistent with extra shielding of the could charges by the increased ions. May is already back to normal (consistent with the end of re- suspension). 12

PG measurement at Kakioka Latitude Longitude 3613'56"N 14011'11"E Main Sub Electrometer Electrostatic sensor type Field mill type Collector Type Water-dropper Mechanical Height 2.55 m 1.00m Separation from the wall 1.17 m Sampling 1 sec 1sec 13

Overview of radioactive deposition 14