E- Donor Bridge Acceptor 1 Acceptor 2 Barrier +· -· -· e-

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e- Donor Bridge Acceptor 1 Acceptor 2 Barrier +· -· -· e-

· +· -· · Radical 1 Donor Bridge Acceptor Radical 2 e-

Time D-B-A1-A2 → D+-B-A1--A2 → D+-B-A1--A2 → D+-B-A1-A2 - π/2 8 ns π Figure 3. Electron transfer pathway (top) and pulse sequence for “J-Jump” experiment. h1 /2-mw h2 D-B-A1-A2 → D+-B-A1--A2 → D+-B-A1--A2 → D+-B-A1-A2 - π/2 8 ns π 16ns 416 nm 7 ns 480 nm Time h /2-mw Figure 5. Electron transfer pathway (top) and pulse sequence for SCRP gated spin information transfer experiment. . R1-D-A-R2 → R1-D-A-R2 → R1-D+-A--R2 R1-D+-A--R2