Rotational and vibrational energy distributions of surface scattered molecules. Rotational and vibrational energy distributions of surface scattered molecules.

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Rotational and vibrational energy distributions of surface scattered molecules. Rotational and vibrational energy distributions of surface scattered molecules. (A) Population distributions of molecules scattered into v = 3, Ω = 0.5 as function of the final rotational energy. Green diamonds show the isotropic distribution (no preferred orientation in the incoming molecular beam); red dots and blue triangles show the rotational distributions obtained with the O-first and N-first orientations, respectively. (B) Same population distributions obtained for the vibrational inelastic channel v = 2, Ω = 0.5. The Inset of A shows the orientation-dependent NO(v = 3) survival probability, P33. The Inset of B shows the relaxation probability to v = 2, P32. Information for these two Insets was obtained from experiments described in the text describing Fig. 5. The black dashed lines show rotational distributions expected for thermalized molecules at room temperature. Bartels N et al. PNAS 2013;110:17738-17743 ©2013 by National Academy of Sciences