Fig. 4 Phonon-polariton laser emission spectra.

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Fig. 4 Phonon-polariton laser emission spectra. Phonon-polariton laser emission spectra. (A) High-resolution emission spectra of the FP devices. The cavity length of all the devices was fixed at 1.0 mm. The longitudinal mode spacing is strongly reduced when the laser emission energy approaches to the AlAs optical phonon energy. The spectral measurements were performed at T = 15 K. (B) Group refractive index (ng) retrieved from the longitudinal mode spacing of the FP devices. The red solid points represent ng of the FP devices containing the AlAs phonon oscillators, while the group index ng of the FP devices without the AlAs phonon oscillators are depicted by the blue solid points (the symbols represent different samples as given in the Supplementary Materials). The red solid line shows ng derived from the computed phonon-polariton dispersion. (C) Computed phonon-polariton dispersion for our laser devices. The red circles represent the emission energies of the measured devices in (B). (D) Computed Hopfield coefficients. In this model, a phonon fraction of 0.65 is obtained at the lowest emission energy (47.2 meV). Keita Ohtani et al. Sci Adv 2019;5:eaau1632 Copyright © 2019 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC).