1 Fusion enhancement due to energy spread of colliding nuclei* 1. Motivation: anomalous electron screening or what else ? 2. Energy spread fusion enhancement 3. Calculate fusion enhancement due to thermal motion of target atoms 4. Generalize to similar processes: - Lattice vibration - Beam energy width - Energy straggling 5. So far, so what? * Work in progress by B Ricci, F Villante and G Fiorentini
2 Anomalous electron screening or what else? At the lowest measured energies, fusion rates are found generally larger than expected, i.e. the enhancement factor f= meas / Bare is: f > f ad where f ad is the maximal screening effect consistent with QM [ In the adiabatic limit energy transfer from electrons to colliding nuclei is maximal ]. Measured values are typically: (f-1) ( ) % for p+d, d+d, d+ 3 He in gas target (f-1) 100% for d+d with d inplanted in metals Are we seeing anomalous screening or something else?
3 Energy spread implies fusion enhancement Consider an example: -The projectile has fixed V -The target has a velocity distribution due (e.g.) to thermal motion: P(v) exp[-v 2 / 2v t 2 ] -Can one neglect the target velocity distribution assuming that “it is zero on average”, i.e.: = (V) ??? NO:Due to strong velocity dependence, approaching particles have larger weight than the receding ones. i f= / (V) >1 V V+v t V-v t
4 Calculation of the effect Generally one has to calculate: f= exp [ v o v t 2 / 2V 4 ] f= / (V) >1 Where is the average over the velocity distribution: f = dv exp [-v o / V-v -v 2 / 2v t 2 ] / exp[- v o /V] dv exp [-v 2 / 2v t 2 ] The calculation can be easily done by a “Gamow trick”. The result is*: where V=proj. vel., v t = target av. thermal vel.,v o =2 Z 1 Z 2 c * We are assuming S=const; for S=S(E) see later…The result is to the leading order in v/V Maxwell vv max
5 Remarks 1. f> 1 i.e. always enhancement Gamow-like peak; largest contribution from target nuclei with: v = v max = v o v t 2 / V 2 f is strongly energy dependent, f exp (-k/ E 2 ). En. Dependence different fromscreening: f sc exp (-k/ E 3/2 ) Effect is small in present conditions: (f-1) for d+d at (c.m.) E = 2 keV It would be significant at extremely low energies: (f-1) 10% for d+d at E = 0.2 keV f= exp [ v o 2 v t 2 / 2V 4 ] V =proj. vel., v t = target av. thermal vel. v o =2 Z 1 Z 2 c
6 Effective energy enhancement If one takes into account that S=S(E) an additional effect arises. The “Gamow peak”means that the S factor is measured for an effective velocity V eff = V(1+ v o v t 2 / V 3) Equivalently, the effective c.m. energy E eff is larger than E=1/2 V 2 : E eff =E (1 + v o v t 2 ( /2E) 3/2 ] 2. The effect can thus be interpreted as an enhancement of the effective collision energy. Really a very tiny effect: for d+d at E CM = 2 keV Maxwell vv max S
7 Correction of S If S exp has been measured at a nominal energy E=1/2 V 2, from: S exp (E) = exp E(V exp (v o /V) in order to obtain the true S factor one has to: - Change to the effective energy E--> E eff -Apply a renormalization factor: S(E eff ) = S exp (E) E exp /E exp [-v o 2 v t 2 / 2V(E) 4 ] S exp (E) S(E eff ) E E eff
8 Generalization to similar processes There are two ingredients in the calculation: exp [ - v o /V rel V rel =relative velocity) P(v) exp [-v 2 / 2v t 2 ] The same scheme can be used for other processes, which produce a (Gaussian) velocity spread of target and/or projectile nuclei. One only has to re-interpret v t 2, by introducing a suitable (v t 2 ) eff f= exp [ v o 2 (v t 2 ) eff / 2V 4 ]
9 Vibrational effects Consider the target nucleus (e.g. d) inplanted in a crystal*). The typical vibrational energies are E vib =(0.1-1) eV Since the collision time is short compared to the vibrational period, one can use the sudden approximation for the target nucleus motion. In the harmonic oscillator approximation, one has: = 1/2 E vib This means = 1/2 (KT) eff (V t 2 ) eff = E vib /m d d *)Similar considerations hold for molecular vibrations
10 Enhancement due Vibrational effects Resulting effects are small: (f-1) 3 ( )for d+d at E CM = 2 keV They can become significant at smaller energy. The value observed for d in some metals, f-1 100%, would correspond to E vib 10 eV d This gives for the enhancement factor: f= exp [ v o 2 vib / 2 m d V 4 ]
11 Beam energy width The produced beam is not really monochromatic: P(E) exp [-(E-E L ) 2 /2 beam ] For LUNA, beam 10 eV. (V t 2 ) eff = beam / 2m p E L This can be transformed into an approximately gaussian velocity distribution with: EELEL ( m p = projectile mass)
12 Enhancement due to Beam energy width Effects are very small in the LUNA condition: (f-1) for d+d at E CM = 2 keV and beam 10 eV The effect behaves quadratically with beam and it can be significant if momentum resolution is worse. EELEL The enhancement factor is thus: f= exp [ v o 2 beam / 2 m 2 p V 6 ]
13 Check As a check, one can show that the same result can be obtained by integrating directly over the energy distribution : P(E) exp [-(E-E L ) 2 /2 beam ] f = / (E L )= exp( v o 2 beam / 2m p 2 V 6 ) By using the saddle point method and assuming beam << E L one finds: EELEL This is the same result as before.
14 Energy loss and straggling Due to atomic collisions in the target one has - Energy loss, E lost - Energy Straggling, stra stra =(E lost ) 1/2 If is the energy lost in each of N collisions E lost stra For E lost 1KeV, 10 eV stra 100 eV. One has the same formula as before, however with stra >> beam : E f = / (E L )= exp( v o 2 E lost / 2m p 2 V 6 )
15 Competition between energy loss and straggling Consider particles entering the target with kin. energy E in. As they advance their kin. energies are decreased. When the average kin. energy is E L =1/2 m p V 2 the correct weight to the cross section is: 1/V 2 exp (v o /V) exp( v o 2 E lost / 2m p 2 V 6 ) The last term is due to straggling. It is: -negliglible at E L E in ( since E lost =0), where most fusions occur. -large at small energies, when fusion is anyhow suppressed. For this reason we expect the effect is not important... E
16 So far, so what ? Energy spread is a mechanism which provides fusion enhancement We have found a general expression for calculating the enhancement f= / due to a gaussian spread: Quantitative estimates for d+d at E cm = 2KeV: thermal(f-1) vibrational(f-1) beam (f-1) No explanation for anomalous screening found; actually we can exclude several potential candidates. f= exp [ v o 2 (v t 2 ) eff / 2V 4 ]