SH nuclei – structure, limits of stability & high-K ground-states/isomers 1.Equilibrium shapes 2.Fission barriers 3.Q alpha of Z=98-126 ( with odd and.

Slides:



Advertisements
Similar presentations
Description of heavy nuclei masses by macro-micro models 1. Coworkers: Yu. Litvinov, A. Parkhomenko 2. Introduction 3. Considered models 4. Accuracy of.
Advertisements

Search for key nuclear structure states below 132 Sn M. Górska, M. Pfützner, H. Grawe et al.
Shell model studies along the N~126 line Zsolt Podolyák.
RFSS: Lecture 4 Alpha Decay
Anatoli Afanasjev Mississippi State University Recent progress in the study of fission barriers in covariant density functional theory. 1. Motivation 2.
Pavel Stránský 29 th August 2011 W HAT DRIVES NUCLEI TO BE PROLATE? Instituto de Ciencias Nucleares, Universidad Nacional Autónoma de México Alejandro.
Isomers and shape transitions in the n-rich A~190 region: Phil Walker University of Surrey prolate K isomers vs. oblate collective rotation the influence.
J.H. Hamilton 1, S. Hofmann 2, and Y.T. Oganessian 3 1 Vanderbilt University, 2 GSI 3 Joint Institute for Nuclear Research ISCHIA 2014.
RADIOACTIVE DECAY NCCS 1.1.4
Kazimierz What is the best way to synthesize the element Z=120 ? K. Siwek-Wilczyńska, J. Wilczyński, T. Cap.
IS THE NUCLEAR LARGE AMPLITUDE COLLECTIVE DYNAMICS ADIABATIC OR NON ADIABATIC ? W. Brodziński, M. Kowal, J. Skalski National Centre for Nuclear Research(Warsaw)
Secondary Minima and Non-axial Saddles in Superheavy (Z around 120) Introduction Method ot the analysis Deformation space Results Summary P. Jachimowicz,
Fusion-Fission Dynamics for Super-Heavy Elements Bülent Yılmaz 1,2 and David Boilley 1,3 Fission of Atomic Nuclei Super-Heavy Elements (SHE) Measurement.
Superdeformed oblate superheavy nuclei - mean field results 1.Introduction – some features of exotic shapes 2.Decay modes & possibility of K-isomers 3.Selfconsistent.
Further microscopic studies of the fission barriers of heavy nuclei T. V. Nhan Hao 1,2) J. Le Bloas 1) M.H. Koh 1,3) L. Bonneau 1) P. Quentin 1) 1) CENBG,
The ground state structure and alpha decay of Hs super- heavy isotopes Junqing Li (Institute of Modern Physics, CAS,Lanzhou) KITPC-CAS Relativistic many-body.
Effect of non-axial deformations of higher multipolarity on the fission-barrier height of heavy and superheavy nuclei I. Introduction II. Method of the.
Fission barriers of heavy and superheavy nuclei analyzed in multidimensional deformation space I.Introduction II.Method III.Deformation space IV.Results.
Systematics of the First 2 + Excitation in Spherical Nuclei with Skyrme-QRPA J. Terasaki Univ. North Carolina at Chapel Hill 1.Introduction 2.Procedure.
Relative kinetic energy correction to fission barriers 1. Motivation 2. Results for A= systems 3. A cluster model perspective 4. Prescription based.
University of Brighton 30 March 2004RISING stopped beam physics workshop Microsecond isomers in A~110 nuclei Few nuclei have oblate ground states (~86%
Single particle properties of heavy and superheavy nuclei. Aleksander Parkhomenko.
Terminating states as a unique laboratory for testing nuclear energy density functional Maciej Zalewski, UW under supervision of W. Satuła Kazimierz Dolny,
ROLE OF THE NON-AXIAL OCTUPOLE DEFORMATION IN THE POTENTIAL ENERGY OF HEAVY AND SUPERHEAVY NUCLEI XVI NUCLEAR PHYSICS WORKSHOP Kazimierz Dolny 23. –
Oscillations in mass asymmetry in second and third minima in actinides 1. Second & third minima in actinides 2. Barrier calculations: Micro-macro vs. selfconsistent.
 What are the appropriate degrees of freedom for describing fission of heavy nuclei (171 ≤ A ≤ 330)?  Fission barrier heights for 5239 nuclides between.
SUPERDEFORMED OBLATE SUPERHEAVY NUCLEI ? SDO minima Stability of SDO nuclei K-isomerism Discussion Summary P. Jachimowicz, M. Kowal, J. Skalski.
Description of experimental fission barriers of heavy nuclei I.Introduction II.Experimental barriers III.Method of description IV.Deformation space V.Results.
1 Alpha Decay Readings §Nuclear and Radiochemistry: Chapter 3 §Modern Nuclear Chemistry: Chapter 7 Energetics of Alpha Decay Theory of Alpha Decay Hindrance.
1 Alpha Decay Energetics of Alpha Decay Theory of Alpha Decay Hindrance Factors Heavy Particle Radioactivity Proton Radioactivity Identified at positively.
M. Girod, F.Chappert, CEA Bruyères-le-Châtel Neutron Matter and Binding Energies with a New Gogny Force.
Nuclear and Radiation Physics, BAU, 1 st Semester, (Saed Dababneh). 1 Nuclear Binding Energy B tot (A,Z) = [ Zm H + Nm n - m(A,Z) ] c 2 B  m.
Nuclear Level Densities Edwards Accelerator Laboratory Steven M. Grimes Ohio University Athens, Ohio.
1 In-Beam Observables Rauno Julin Department of Physics University of Jyväskylä JYFL Finland.
Shape phase transition in neutron-rich even-even light nuclei with Z=20-28 H.B.Bai X.W.Li H.F.Dong W.C.Cao Department of Physics, Chifeng University, Chifeng.
Nuclear structure theory of the heaviest nuclei: achievements and challenges. Anatoli Afanasjev Mississippi State University 1.Introduction 2.Actinides.
Ning Wang 1, Min Liu 1, Xi-Zhen Wu 2, Jie Meng 3 Isospin effect in Weizsaecker-Skyrme mass formula ISPUN14, , Ho Chi Minh City 1 Guangxi Normal.
Kazimierz 2011 T. Cap, M. Kowal, K. Siwek-Wilczyńska, A. Sobiczewski, J. Wilczyński Predictions of the FBD model for the synthesis cross sections of Z.
The excitation and decay of nuclear isomers Phil Walker CERN and University of Surrey, UK 3. Isomers at the limits of stability ● p decay ● n decay ● α.
Coupling of (deformed) core and weakly bound neutron M. Kimura (Hokkaido Univ.)
ESNT Saclay February 2, Structure properties of even-even actinides at normal- and super-deformed shapes J.P. Delaroche, M. Girod, H. Goutte, J.
Erosion of N=28 Shell Gap and Triple Shape Coexistence in the vicinity of 44 S M. KIMURA (HOKKAIDO UNIV.) Y. TANIGUCHI (RIKEN), Y. KANADA-EN’YO(KYOTO UNIV.)
Ning Wang An improved nuclear mass formula Guangxi Normal University, Guilin, China KITPC , Beijing.
Deformations of sd and pf shell  hypernuclei with antisymmetrized molecular dynamics Masahiro Isaka (RIKEN)
Quantum Phase Transitions (QPT) in Finite Nuclei R. F. Casten June 21, 2010, CERN/ISOLDE.
Lecture 21: On to Finite Nuclei! 20/11/2003 Review: 1. Nuclear isotope chart: (lecture 1) 304 isotopes with t ½ > 10 9 yrs (age of the earth) 177.
Shell structure: ~ 1 MeV Quantum phase transitions: ~ 100s keV Collective effects: ~ 100s keV Interaction filters: ~ keV Binding energies, Separation.
Ways to treat spontaneous & other fission from instanton perspective with some results obtained with: W. Brodziński, P. Jachimowicz, M. Kowal, J. Skalski.
WHY ARE NUCLEI PROLATE:
Shape evolution of highly deformed 75 Kr and projected shell model description Yang Yingchun Shanghai Jiao Tong University Shanghai, August 24, 2009.
First Gogny conference, TGCC December 2015 DAM, DIF, S. Péru QRPA with the Gogny force applied to spherical and deformed nuclei M. Dupuis, S. Goriely,
S. L. Tabor – Florida State University ATLAS Users Meeting August 8, 2009 Sam Tabor - Florida State University Intruder states approaching the Island of.
F. C HAPPERT N. P ILLET, M. G IROD AND J.-F. B ERGER CEA, DAM, DIF THE D2 GOGNY INTERACTION F. C HAPPERT ET AL., P HYS. R EV. C 91, (2015)
Quantum phase transitions and structural evolution in nuclei.
Global fitting of pairing density functional; the isoscalar-density dependence revisited Masayuki YAMAGAMI (University of Aizu) Motivation Construction.
Time dependent GCM+GOA method applied to the fission process ESNT janvier / 316 H. Goutte, J.-F. Berger, D. Gogny CEA/DAM Ile de France.
g-ray spectroscopy of the sd-shell hypernuclei
Congresso del Dipartimento di Fisica Highlights in Physics –14 October 2005, Dipartimento di Fisica, Università di Milano Contribution to nuclear.
Current Status of Nuclear Mass Formulae 1 RIBF-ULIC-Symposium: Physics of Rare-RI Ring, RIKEN, Nov , 2011 Hiroyuki KOURA Advanced Science Research.
Pairing Evidence for pairing, what is pairing, why pairing exists, consequences of pairing – pairing gap, quasi-particles, etc. For now, until we see what.
超重原子核的结构 孙 扬 上海交通大学 合作者:清华大学 龙桂鲁, F. Al-Khudair 中国原子能研究院 陈永寿,高早春 济南,山东大学, 2008 年 9 月 20 日.
Emmanuel Clément IN2P3/GANIL – Caen France
Study of SHE at the GSI – SHIP
Nuclear masses of neutron-rich nuclei and symmetry energy
From instantons to spontaneous fission rates
a non-adiabatic microscopic description
Symmetry energy coefficients and shell gaps from nuclear masses
Superheavy nuclei: relativistic mean field outlook
An improved nuclear mass formula
Presentation transcript:

SH nuclei – structure, limits of stability & high-K ground-states/isomers 1.Equilibrium shapes 2.Fission barriers 3.Q alpha of Z= ( with odd and odd- odd) nuclei. 4.K-isomers or high–K ground states of odd & odd-odd nuclei - a chance for longer half- lives 5. Predictions for SHE with Z>126 P.Jachimowicz (UZ), W.Brodziński, M.Kowal, J.Skalski (NCBJ) ARIS 2014, Tokyo, Japan Mostly results of the Woods-Saxon micro-macro model; some Skyrme HFBCS results.

Ground state shapes, even-even Micro-macro results In contrast to many Skyrme forces, Woods-Saxon micro- macro model gives lower barriers and mostly oblate ground states for Z>=124,126 (no magic gap for 126 protons). P. Jachimowicz, M. Kowal, and J. Skalski, PRC 83, (2011).

SLy4, M. Bender, P-H. Heenen, to be published (inverted colors) Gogny force, M. Warda L. Próchniak

Possible alpha-decay hindrance: the 14- SD oblate ground state in parent. The G.S. to G.S. transition inhibited; SDO to SDO has the Q value smaller by 2 MeV.

Fission barriers calculated using micro- macro model (e-e nuclei) Performance for even-even actinides: 1-st barriers, 18 nuclei rms : 0.5 MeV 2-nd barriers, 22 nuclei rms : 0.69 MeV Even-even SH nuclei: barries decrease for Z>114 The highest barrier for Z=114, N=178 P. Jachimowicz, M. Kowal, and J. Skalski, PRC 85, (2012). M. Kowal, P. Jachimowicz and A. Sobiczewski, PRC 82, (2010).

Heaviest even-even fissioning nuclei: 112, ms (old calc. 71 ms) 112, ms (old calc. 4 s) 114, ms (old calc. 1.5 s) (for Z=114, the local minimum in barrier at N=168) Old calculation: Smolańczuk, Skalski, Sobiczewski (1995)

HN – Woods-Saxon FRLDM – P. Moller et al. SkM* - A.Staszczak et al. RMF – H.Abusara et al. FRDLM & RMF also perform well in actinides! Comparison of various models: some must be wrong.

SHE masses (including odd & odd-odd) A fit to exp. masses Z>82, N>126, number of nuclei: 252 For odd and odd-odd systems there are 3 additional parameters – macroscopic energy shifts (they have no effect on Q alpha). >>Predictions for SHE: 88 Q alpha values, Z= , 7 differ from exp. by more than 0.5 MeV; the largest deviation: 730 keV (blocking). Slight underestimate for Z=108; Overestimate: Z= P. Jachimowicz, M. Kowal, and J. Skalski, PRC 89, (2014)

Statistical parameters of the fit to masses in the model with blocking in separate groups of even- even, odd-even, even-odd and odd-odd heavy nuclei: The same but for the method without blocking. Q alpha 204 nuclei in the fit region blocking q.p.method mean 326 keV 225 keV error rms 426 keV 305 keV 88 nuclei Z= mean 217 keV 196 keV error rms 274 keV 260 keV

High-K states: a chance for longer half-lives. < Candidates for high-K g.s. in odd or odd-odd SHN in the W-S model In even-even systems one should block high-K close-lying orbitals, like: 9/2+ and 5/2- protons below Z=108 or 11/2- and 9/2+ neutrons below N=162 Z N Omega(n) Omega(p) K /2+ 7/ /2- 15/ /2+ 11/ /2+ 9/ /2- 3/ /2- 13/ All 11/2+ > 11/ /2+ „ „ „ „ 159 „ „ „ /2- „ „ 13/ /2- 11/ /2- 5/ /2- „ /2- 13/ /2- 11/ /2- 9/ /2- 9/ /2- 11/ /2- 7/ /2- 7/ /2+ 7/ /2- 1/2- 6+

protons

neutrons

Unique blocked orbitals may hinder alpha transitions. The effect of a reduced Q alpha for g.s. -> excited state (left panel) on the life-times (below) according to the formula by Royer.

G.S. configuration: P:11/2+ [6 1 5] N:13/2- [7 1 6] Fixing the g.s. configuration rises the barrier by 6 MeV. Even if configuration is not completely conserved, a substantial increase in fission half-life is expected.

Microscopic-macroscopic method Shape parametrization: β 20 & β 22 on the mesh, minimalization in {β 40 β 60 β 80 β 42 β 44 }. Hartree-Fock-BCS with SLy6 force – an „upper limit” for barrier 180 neutron & 110 proton levels Pairing: delta interaction of time-reversed pairs with a smooth energy cutoff, V n = 316 MeV fm 3, V p = 322 MeV fm 3 Stability for Z>126 W. Brodziński, J. Skalski, Phys. Rev C 88, (2013)

Macroscopic energy vs axial elongation in the beta-gamma plane

Spherical shell correction with the SLy6 force; W-S gives a very similar pattern for Z>126

In both W-S and SLy6 models -doubly magic spherical system. In the W-S model: Q alpha = 14.3 MeV. From the formula by Royer et al. T alpha = 100 s. B eff > 700 hbar^2/MeV, along a stright path (axially symmetric) one obtains T fission > 10^7 s. Next doubly magic nucleus??

β-stable, HFBCS: Q α ≈10 MeV, T alpha = 0.1 s, T fission (rough estimate) = 10^{-6} s; more for odd & odd-odd systems W-S minimum: SD-oblate Fission barrier: 2 MeV HFBCS minimum: spherical/SD- Oblate, fission barrier: 4.2 MeV Micro-macroHartree-Fock-BCS N=228 region:

W-S micro-macro model predicts reasonable barriers for actinides and SH nuclei; Q alpha also seem reasonable; Large differences in barriers between our model and the FRDLM or Skyrme-type; nobody knows what happens for Z>=120; High-K ground states of some odd and odd-odd nuclei, with blocked intruder orbitals, may be the longest-lived SHE; Z>126 systems – rather pessimistic predictions: nonaxiality ruins stability; no stability in the W-S model, while SLy6, known to give too high barriers (by up to 2.5 MeV), leads to estimated (roughly) fission half-lives:10^-6 s & alpha half-lives of 0.1 s. This does not promise much stability. Conclusions