Perspectives on Long Range Transport – Jeff Lundgren and Ian McKendry Geog/ATSC UBC

Emerging interest on West Coast and elsewhere in Chemical Weather : “ local, regional and global distributions of important trace gases and aerosols and their variabilities on time scales of minutes to hours to days, particularly in light of their various impacts, such as on human health, ecosystems, and the meteorological weather and climate”. - Lawrence et al

Outline History – a West Coast Perspective History – a West Coast Perspective Trans-Pacific Transport – what we know Trans-Pacific Transport – what we know Defining “Background” and “chemical weather” - importance to Canada Wide Standards Defining “Background” and “chemical weather” - importance to Canada Wide Standards Outstanding scientific issues Outstanding scientific issues

Chernobyl 1986 alerted us to potential impacts of Long Range Transport

Evidence from West of LRT – Siberian Fires etc. McKendry and Lundgren 2000 Climatology of Layer Structures

1998 Asian Dust Event was the catalyst for research a. GOES 10 geostationary satellite image of the dust taken on the evening of April 27. The dust cloud, marked by the brighter reflectance covers the entire northwestern US and adjacent portions of Canada. A dust stream is also seen crossing the Rocky Mountains toward the east. b. Contour map of the PM10 concentration on April 29, Note the coincidence of high PM10 and satellite reflectance over Washington c. Regional average daily PM10 concentration over the West Coast. The sharp peak on April is due to the Asian dust.

On Heels of 1998 Event came April : “The Perfect Asian Dust Storm”

Jaffe et. al. ongoing Aircraft and monitoring in Western North America highlights diversity and frequency of events Jaffe et al. 2003

Dust Veils streaming off North Africa 1 March 2005 (this image from the Moderate Resolution Imaging Spectroradiometer (MODIS) on NASA’s Terra satellite). Available online at the NASA Earth Observatory: tp://earthobservatory.nasa.gov/NaturalHazards/ (MODIS)Terra(MODIS)Terra 2005: A New Pathway identified for Dust – Sahara Eastward to North America

GEOS-CHEM Model Note lack of dust activity near surface Over Eurasia and No precipitation En route ~19,000km

EC Lidar at UBC March 2005

A B NRL Aerosol Forecast for Saturna Is. Saharan Dust Layer Cloud Lidar Backscatter

A B NRL Aerosol Forecast for Saturna Is. Lidar Backscatter Subsidence

Spring Zonal fluxes  gm -2 s -1 at 140 o W Gong et al From Sunling Gong’s work we know a lot now about the Inter-annual variability and pathways of Asian LRT

A novel approach to investigating transport – tremendous potential Mean Asian transit time 8 days in mid-trop And 14 days at surface

Scales and Processes affecting intercontinental transport Subsidence Synoptic systems Local winds Boundary layer Processes Chemistry SOURCESINK TRANSPORT Convection Synoptic systems Boundary Layer Warm Conveyer Belts Planetary waves Deposition Processes Chemistry Synoptic “handover” Minutes - days ~10-15 days Minutes-days

Objectives of Ongoing Research Identify global pathways Identify global pathways Climatology of transport pathways Climatology of transport pathways Estimate burden Estimate burden Identify trends Identify trends Estimate contribution to local air quality Estimate contribution to local air quality

background concentration (level) is formally defined as: “The concentration of a given species in a pristine air mass in which anthropogenic impurities of a relatively short lifetime are not present. The background concentrations of relatively long-lived molecules, methane, carbon dioxide, halocarbons (CF3Cl, CF2Cl2, etc.) and some other species continue to rise due to anthropogenic input, so the composition of background air is undergoing continual change. Background concentration of a given species is sometimes considered to be the concentration of that impurity in a given air mass when the contribution from anthropogenic sources under study is absent. Synonymous with baseline concentration.” 1990, 62, 2175 IUPAC Compendium of Chemical Terminology 2nd Edition (1997) Estimating contribution to local air quality: With the move to Canada Wide Standards for PM 2.5 and O 3 there is a need to define background concentrations that not amenable to control strategies and may violate standards

GFDL Modelling

Keating et al 2005

Keating et al. 2005

NOTE: Proposed CWS PM 2.5 : 30  gm- 3, 24-hour (midnight to midnight) averaging time - 98th percentile ambient measurement annually, averaged over three consecutive years. (Combined Marine Asian Air)

Impact of Episodic events (“Chemical Weather”) on PM 2.5 Background Maximum ambient PM 2.5 Concentration Duration of Event Background contribution to ambient Spatial ExtentFrequency Kelowna August 2003 Forest Fires 284 µgm -3 7 days100% Regionalinterannual April 1998 Asian Dust Event 1 44µgm -3 days50% 2 Continentalrare (decadal?) Chilliwack local dust event (7 Jan 2005) 2-5µgm -3 (PM 10 50µgm -3 ) days0-50% Localannual 1 McKendry et al, 2001; Husar et al EPA (2002) suggest an increase of 8.7± 2.3 µgm -3 during dust events, with mean maximum dust contributions of 19.7± 8.4 µgm -3

Scientific Issues Multiple phenomena occurring across a range of spatial and temporal scales Multiple phenomena occurring across a range of spatial and temporal scales Events singular (spring maximum) Events singular (spring maximum) Observations are difficult and interpretation involves multiple lines of evidence Observations are difficult and interpretation involves multiple lines of evidence Chemistry likely complex Chemistry likely complex Urgent need for continuous lidar measurements on west Coast to complement Whistler High Altitude measurements Urgent need for continuous lidar measurements on west Coast to complement Whistler High Altitude measurements

Publications McKendry, I. G. and J. Lundgren, "Tropospheric layering of ozone in regions of urbanised complex and/or coastal terrain - a review," Progress in Physical Geography, 24, p McKendry, I. G. and J. Lundgren, "Tropospheric layering of ozone in regions of urbanised complex and/or coastal terrain - a review," Progress in Physical Geography, 24, p McKendry, I. G., J. P. Hacker, R. Stull, S. Sakiyama, D. Mignacca and K. Reid, "Long range transport of Asian dust to the Lower Fraser Valley, British Columbia, Canada," Journal of Geophysical Research, 106(D16), p McKendry, I. G., J. P. Hacker, R. Stull, S. Sakiyama, D. Mignacca and K. Reid, "Long range transport of Asian dust to the Lower Fraser Valley, British Columbia, Canada," Journal of Geophysical Research, 106(D16), p Husar, R. B., D. M. Tratt, B. A. Schichtel, S. R. Falke, F. Li, D. Jaffe, S. Gassó, T. Gill, N. S. Laulainen, F. Lu, M. C. Reheis, Y. Chun, D. Westphal, B. N. Holben, C. Gueymard, I. McKendry, N. Kuring, G. C. Feldman, C. McClain, R. J. Frouin, J. Merrill, D. DuBois, F. Vignola, T. Murayama, S. Nickovic, W. E. Wilson, K. Sassen, N. Sugimoto and W. C. Malm, "The Asian dust events of April 1998," Journal of Geophysical Research, 106(D16), p Husar, R. B., D. M. Tratt, B. A. Schichtel, S. R. Falke, F. Li, D. Jaffe, S. Gassó, T. Gill, N. S. Laulainen, F. Lu, M. C. Reheis, Y. Chun, D. Westphal, B. N. Holben, C. Gueymard, I. McKendry, N. Kuring, G. C. Feldman, C. McClain, R. J. Frouin, J. Merrill, D. DuBois, F. Vignola, T. Murayama, S. Nickovic, W. E. Wilson, K. Sassen, N. Sugimoto and W. C. Malm, "The Asian dust events of April 1998," Journal of Geophysical Research, 106(D16), p Hacker, J. P., I. G. McKendry and R. B. Stull, "Modeled downward transport of Asian dust over Western North America during April 1998," Journal of Applied Meteorology, 40, p Hacker, J. P., I. G. McKendry and R. B. Stull, "Modeled downward transport of Asian dust over Western North America during April 1998," Journal of Applied Meteorology, 40, p D. Jaffe, I. G. McKendry and H. Price "Six Case Studies of Trans-Pacific Transport of Air Pollutants," Atmospheric Environment, 37, D. Jaffe, I. G. McKendry and H. Price "Six Case Studies of Trans-Pacific Transport of Air Pollutants," Atmospheric Environment, 37, S. L. Gong, X. Y. Zhang, T. L. Zhao, I. G. McKendry and D. Jaffe “Characterization of soil dust aerosol in China and its transport/distribution Journal Geophysical Research. 108(D9) S. L. Gong, X. Y. Zhang, T. L. Zhao, I. G. McKendry and D. Jaffe “Characterization of soil dust aerosol in China and its transport/distribution Journal Geophysical Research. 108(D9) T.L. Zhao, S.L. Gong, X.Y. Zhang, I.G. McKendry 2003, “Modelled size-segregated budgets of soil dust aerosol during ACE-Asia, 2001: Implications for Trans-Pacific transport” - Journal of Geophysical Research, 108, D23, T.L. Zhao, S.L. Gong, X.Y. Zhang, I.G. McKendry 2003, “Modelled size-segregated budgets of soil dust aerosol during ACE-Asia, 2001: Implications for Trans-Pacific transport” - Journal of Geophysical Research, 108, D23, H. Price, D. Jaffe, P. Doskey, I. McKendry and T. Anderson. 2003: “Vertical Profiles of O3, aerosols, CO and NMHCs in the Northeast Pacific during the ACE-ASIA and TRACE-P experiments” J. Geophys. Res.Vol. 108, No. D20, 8799 H. Price, D. Jaffe, P. Doskey, I. McKendry and T. Anderson. 2003: “Vertical Profiles of O3, aerosols, CO and NMHCs in the Northeast Pacific during the ACE-ASIA and TRACE-P experiments” J. Geophys. Res.Vol. 108, No. D20, 8799 M. Holzer, I. G. McKendry and D. Jaffe, 2003 "Springtime trans-Pacific atmospheric transport from East Asia: A transit-time-PDF approach" Journal of Geophysical Research, 108 D22, M. Holzer, I. G. McKendry and D. Jaffe, 2003 "Springtime trans-Pacific atmospheric transport from East Asia: A transit-time-PDF approach" Journal of Geophysical Research, 108 D22, Zhao, T.L., S. L. Gong, X. Y. Zhang, I. G. McKendry, and Z. J. Zhou 2006 “A Simulated Climatology of Asian Dust Aerosol and its Trans-Pacific Transport 1. Mean climate and validation” J. Climate 19(1): Zhao, T.L., S. L. Gong, X. Y. Zhang, I. G. McKendry, and Z. J. Zhou 2006 “A Simulated Climatology of Asian Dust Aerosol and its Trans-Pacific Transport 1. Mean climate and validation” J. Climate 19(1): Gong, S.L., X.Y. Zhang, T.L. Zhao, X. Zhang, I.G. McKendry and C.S. Zhao. 2006: “A Simulated Climatology of Asian Dust Aerosol and its Trans-Pacific Transport 2. Interannual Variability and Climate Connections”, J. Climate 19(1): Gong, S.L., X.Y. Zhang, T.L. Zhao, X. Zhang, I.G. McKendry and C.S. Zhao. 2006: “A Simulated Climatology of Asian Dust Aerosol and its Trans-Pacific Transport 2. Interannual Variability and Climate Connections”, J. Climate 19(1): Bennett C.M., I.G. McKendry, S. Kelly, K. Denike and T. Koch “Impact of the 1998 Gobi Dust Event on Hospital Admissions in the Lower Fraser Valley, British Columbia”, Science of the Total Environ. (in Press) Bennett C.M., I.G. McKendry, S. Kelly, K. Denike and T. Koch “Impact of the 1998 Gobi Dust Event on Hospital Admissions in the Lower Fraser Valley, British Columbia”, Science of the Total Environ. (in Press) McKendry, Strawbridge, O’Neill, McDonald, Liu, P. Jaegle, Jaffe, Fairlie, A Case of Trans-Pacific Transport of Saharan Dust to Western North America, JGR McKendry, Strawbridge, O’Neill, McDonald, Liu, P. Jaegle, Jaffe, Fairlie, A Case of Trans-Pacific Transport of Saharan Dust to Western North America, JGR