10/28/2014 Xiangshang Li, Yunsoo Choi, Beata Czader Earth and Atmospheric Sciences University of Houston The impact of the observational meteorological.

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10/28/2014 Xiangshang Li, Yunsoo Choi, Beata Czader Earth and Atmospheric Sciences University of Houston The impact of the observational meteorological nudging and nesting on the simulated meteorology and ozone concentrations from WRF-SMOKE-CMAQ during DISCOVER-AQ 2013 Texas campaign

UH Air Quality Forecasting (12km & 4km) University of Houston

September 2013 Four complete set of WRF-SMOKE-CMAQ simulations; new model version and 2008 inventory 12km Chemical boundary condition is used Detailed analyses – Variables Meteorology: T/U/V/CFRAC/CLDT/TEMP2/PBL Chemistry: Ozone/NO/NO 2 /NOx/Isoprene etc DISCOVER-AQ Simulation University of Houston

Analyses – Various satellite cloud, radar images and weather charts – Hourly precipitation data – Full statistics (CORR, IOA, MB, MAE etc) for major variables (T/U/V/O 3 /NO/NO 2 /NOx) Daily By site Day-time Night-time – Spatial and time-series plots – High ozone episode due to front passage (09/25-09/26) – Inland and coastal sites – Background ozone – Bogus thunderstorms DISCOVER-AQ Simulation University of Houston

Satellite Visible – _11 CST Radar – _11 CST

Ozone at La Porte Wind progression on sites at Houston

09/25 high ozone day: 10 CST University of Houston

Model missed the high ozone around La Porte: 13 CST University of Houston High ozone Bay breeze fully developed

Land/Sea/Bay breeze etc University of Houston Land breeze and sea/bay breeze Local wind reversal, convergence Small-scale phenomenon, short life time, a few hours Occurs when large scale forcing is absent -> prone to high ozone Extremely important for simulating high ozone episode Hard for WRF to replicate

Observation nudging University of Houston FDDA is one of the most important components in modern NWP models Model performance gain is substantial while cost is relatively low Nudging is a FDDA method to push (or nudge) model values toward observation. – Grid nudging uses analysis input (‘met_em’ files from WPS) – Obs-nudging uses observation data (OBS_DOMAIN files from WRF-OBSGRID) Obs-nudging is performed every 3 hours, just like the grid nudging Time Nudging Improvement of IOA: Wind (U and V) 10-14%; Temperature 9%

Improvement significant

WRF Obs nudging – op. flow chart

OA did not solve the problem for 09/25 University of Houston No bay breeze

Current work: Enhanced obs nudging University of Houston In 09-25, last nudging is performed at 9 CST, yet baybreeze onset is at 10 CST – From 10 to 13 CST, there is only one nudging done at 12 CST -> Not enough push to ‘bend’ model! Possible solution – Increase the obs nudging frequency to hourly! Data available, already preprocessed WRF does not support it – Implementation – First task (modifying OBSGRID code) done! – On 2 nd task (modifying WRF)

High CMAQ background Ozone University of Houston High ozone bias ~ 7-8 ppb Possible Cause – Coastal sites such as Galveston (C1034) have higher biases, the most inland site (C78 Conroe) has very small bias – Production is typically low at C1034 – Suggesting model background ozone may be a factor since prevailing winds are from southeast

CMAQ Background Ozone University of Houston Galveston ozone time series – high bias for many days Model southeast corner time series – pattern similar to C1034 Reducing CMAQ boundary ozone values may help bias reduction

Conclusions University of Houston Different met data produces ozone differences Objective Analysis makes better met data (not all the times) Incapability to capture sea-breeze on Sep 25, 2013 may cause low simulated high ozone 3-hour observation update frequency is not good enough to capture sea-/land-breeze – 1-hour observation update tool needs Ozone is overestimated in the model particularly in Galveston and high overestimated chemical boundary condition may contribute overpredictions