Millimeter Wave Spectroscopy of Cold 85 Rb Atoms JIANING HAN, YASIR JAMIL, PAUL TANNER, DON NORUM, T. F. GALLAGHER University of Virginia Supported by:

Slides:



Advertisements
Similar presentations
High-resolution spectroscopy with a femtosecond laser frequency comb Vladislav Gerginov 1, Scott Diddams 2, Albrecht Bartels 2, Carol E. Tanner 1 and Leo.
Advertisements

First Year Seminar: Strontium Project
Zero-Phonon Line: transition without creation or destruction of phonons Phonon Wing: at T = 0 K, creation of one or more phonons 7. Optical Spectroscopy.
Vibrational Spectroscopy of Cold Molecular Ions Ncamiso Khanyile Ken Brown Lab School of Chemistry and Biochemistry June 2014.
Tunable Laser Spectroscopy Referenced with Dual Frequency Combs International Symposium on Molecular Spectroscopy 2010 Fabrizio Giorgetta, Ian Coddington,
Results The optical frequencies of the D 1 and D 2 components were measured using a single FLFC component. Typical spectra are shown in the Figure below.
Samansa Maneshi, Jalani Kanem, Chao Zhuang, Matthew Partlow Aephraim Steinberg Department of Physics, Center for Quantum Information and Quantum Control,
Selective population of Core Nonpenetrating Rydberg states David Grimes, Yan Zhou, Timothy J Barnum, Ethan Klein, Robert Field Department of Chemistry,
P. Cheinet, B. Pelle, R. Faoro, A. Zuliani and P. Pillet Laboratoire Aimé Cotton, Orsay (France) Cold Rydberg atoms in Laboratoire Aimé Cotton 04/12/2013.
An STM Measures I(r) Tunneling is one of the simplest quantum mechanical process A Laser STM for Molecules Tunneling has transformed surface science. Scanning.
Excitation processes during strong- field ionization and dissociatation of molecules Grad students: Li Fang, Brad Moser Funding : NSF-AMO November 29,
Rydberg physics with cold strontium James Millen Durham University – Atomic & Molecular Physics group.
Dynamical Localization and Delocalization in a Quasiperiodic Driven System Hans Lignier, Jean Claude Garreau, Pascal Szriftgiser Laboratoire de Physique.
MQDT analysis James Millen. Introduction MQDT analysis – Group meeting 13/09/10 In our experiment we measure the population of Rydberg states using autoionization.
Rydberg excitation laser locking for spatial distribution measurement Graham Lochead 24/01/11.
The story unfolds… James Millen The story unfolds… – Group meeting 12/04/10.
Ultraslow Dissociation of H 2 + Via Intense Laser Pulses Presented by: Brad Moser And George Gibson DAMOP 2010.
Autoionization of strontium Rydberg states
1 09:05-09:55 am, Wednesday, September 22, 2010 CHEM 8152: Analytical Spectroscopy Smith 1111, University of Minnesota Resonant cavities Gain Threshold.
Excited state spatial distributions Graham Lochead 20/06/11.
UCLA The X-ray Free-electron Laser: Exploring Matter at the angstrom- femtosecond Space and Time Scales C. Pellegrini UCLA/SLAC 2C. Pellegrini, August.
A strontium detective story James Millen Strontium detective – Group meeting 19/10/09 Ions‽
Stefan Truppe MEASUREMENT OF THE LOWEST MILLIMETER- WAVE TRANSITION FREQUENCY OF THE CH RADICAL.
Single atom lasing of a dressed flux qubit
Physical Phenomena for TeraHertz Electronic Devices
N. Yugami, Utsunomiya University, Japan Generation of Short Electromagnetic Wave via Laser Plasma Interaction Experiments US-Japan Workshop on Heavy Ion.
Accurate density measurement of a cold Rydberg gas via non-collisional two-body process Anne Cournol, Jacques Robert, Pierre Pillet, and Nicolas Vanhaecke.
Progress towards laser cooling strontium atoms on the intercombination transition Danielle Boddy Durham University – Atomic & Molecular Physics group.
Elastic collisions. Spin exchange. Magnetization is conserved. Inelastic collisions. Magnetization is free. Magnetic properties of a dipolar BEC loaded.
Interaction of laser pulses with atoms and molecules and spectroscopic applications.
Analysis of strongly perturbed 1 1  – 2 3  + – b 3  states of the KRb molecule J. T. Kim 1, Y. Lee 2, and B. Kim 3 1 Department of Photonic Engineering,
Quantum interference phenomenon Quantum interference phenomenon in the cold atomic cascade system $$ : National Science Council and National Space Program.
TALKING DIRECTLY TO RYDBERG STATES Yan Zhou, David Grimes, Ethen Klein, Timothy Barnum, Robert Field laser mmW.
Relativistic nonlinear optics in laser-plasma interaction Institute of Atomic and Molecular Sciences Academia Sinica, Taiwan National Central University,
Femtosecond Laser Spectroscopy of C 60 Nieuwegein, The Netherlands August 21, 2001 Eleanor Campbell, Göteborg University & Chalmers, Sweden R.D. Levine,
W I S S E N T E C H N I K L E I D E N S C H A F T  Januar 13 Name und OE, Eingabe über > Kopf- und Fußzeile.
Sanghamitra Deb, Michael P. Minitti, Peter M. Weber Department Of Chemistry Brown University 64 th OSU International Symposium on Molecular Spectroscopy.
Resonant dipole-dipole energy transfer from 300 K to 300μK, from gas phase collisions to the frozen Rydberg gas K. A. Safinya D. S. Thomson R. C. Stoneman.
Enhancing the Macroscopic Yield of Narrow-Band High-Order Harmonic Generation by Fano Resonances Muhammed Sayrac Phys-689 Texas A&M University 4/30/2015.
Excited state spatial distributions in a cold strontium gas Graham Lochead.
Temperature and sample dependence of spin echo in SiC Kyle Miller, John Colton, Samuel Carter (Naval Research Lab) Brigham Young University Physics Department.
Optically detected magnetic resonance of silicon vacancies in SiC Kyle Miller, John Colton, Samuel Carter (Naval Research Lab) Brigham Young University.
Nonlinear optical effect in the soft x-ray region by two-photon ionization of He + Nonlinear optical effect in the soft x-ray region by two-photon ionization.
High resolution spectroscopy with a femtosecond laser frequency comb
Refractive Index Enhancement in Atomic Vapors Deniz Yavuz, Nick Proite, Brett Unks, Tyler Green, Dan Sikes Department of Physics, University of Wisconsin.
Spatial distributions in a cold strontium Rydberg gas Graham Lochead.
Transient enhancement of the nonlinear atom-photon coupling via recoil-induced resonances: Joel A. Greenberg and Daniel. J. Gauthier Duke University 5/22/2009.
Rydberg States of Two Valence Electron Atoms W. E Cooke K.A. Safinya W. Sandner F. Gounand P. Pillet N. H. Tran R. Kachru R. R. Jones.
Spatial distributions in a cold strontium Rydberg gas Graham Lochead.
Toward the use of Rydberg states for state-selective production of molecular ions David Grimes, Timothy J Barnum, Stephen Coy, Robert Field Department.
Broadband Microwave Spectroscopy to Study the Structure of Odorant Molecules and of Complexes in the Gas Phase Sabrina Zinn, Chris Medcraft, Thomas Betz,
Rydberg Series of C 60 Osnabrück, Germany March 2002 Eleanor Campbell, Göteborg University & Chalmers, Sweden R.D. Levine, Fritz Haber Center, Hebrew University.
Theory for Direct Frequency-Comb Spectroscopy Daniel Felinto and Carlos E.E. López 65 th International Symposium on Molecular Spectroscopy June 24, 2010.
Production of vibrationally hot H 2 (v=10–14) from H 2 S photolysis Mingli Niu.
Direct Observation of Rydberg–Rydberg Transitions in Calcium Atoms K. Kuyanov-Prozument, A.P. Colombo, Y. Zhou, G.B. Park, V.S. Petrović, and R.W. Field.
Rydberg atoms part 1 Tobias Thiele.
Microwave Spectroscopy of the Autoionizing 5d 3/2 n l States of Barium Edward Shuman Tom Gallagher.
Multi-step and Multi-photon Excitation Studies of Group-IIB Elements
Microwave Transitions Between Pair States Composed of Two Rb Rydberg Atoms Jeonghun Lee Advisor: Tom F. Gallagher Department of Physics, University of.
Many-Body Effects in a Frozen Rydberg Gas Feng zhigang
Chao Zhuang, Samansa Maneshi, XiaoXian Liu, Ardavan Darabi, Chris Paul, Luciano Cruz, and Aephraim Steinberg Department of Physics, Center for Quantum.
TC, U. Dorner, P. Zoller C. Williams, P. Julienne
Manipulating Rydberg Atoms with Microwaves
Resonant dipole-dipole energy transfer
Coherence & Quantum Technology
Metastable States Arising from the Ablation of Solid Copper
State evolution in cold helium Rydberg gas
Energy diagrams and orientation distributions of the NO molecule.
Resolution of Transient States of Nitrile Anions via Photodissociation Action Spectroscopy; Our Progress to Date The 2 traces show resonant Cu atomic.
Quantum phase magnification
Presentation transcript:

Millimeter Wave Spectroscopy of Cold 85 Rb Atoms JIANING HAN, YASIR JAMIL, PAUL TANNER, DON NORUM, T. F. GALLAGHER University of Virginia Supported by: the Air Force Office of Scientific Research

Outline Motivation Quantum defects measurements Population transfer Conclusion

Motivation Cold rydberg atoms Artificial amorphous solids Automatically evolve into plasma Microwave High resolution spectral probe Manipulate atoms [1] H. Maeda, et al., Science 307, 1757 (2005) Cold rydberg atoms Artificial amorphous solids Automatically evolve into plasma Microwave High resolution spectral probe Manipulate atoms [1] H. Maeda, et al., Science 307, 1757 (2005)

Theory Hydrogen atom: Core polarizationOrbital Penetration Alkali atoms:

The energy diagram and timing T(μs) 480nm dye laser pulse Microwave pulse Field ionization ramp Timing ~480nm 5p 3/2 (n+2)d 5/2 nf Microwave Energy diagram J 5/2 7/2

Selective Field Ionization (SFI) Time Voltage Field ionization ramp Oscilloscope trace

A typical resonance The line width is about the transform limit of a 5 μs microwave pulse The side peaks are the off resonance excitation of a π pulse The 32d 5/2 -30f 7/2 resonance. The microwave pulse length is about 5μs. 200kHz

Results The quantum defects of f 5/2,7/2 states were fitted to the function: The improved and previous quantum defects are listed in table 1

Results If we fit the fine structure intervals between the f 5/2 and f 7/2 by the following function: A = (25)GHz; B = 1.917(13)THz. The fine structure plots. The small plot is a magnified plot for n*>29. The first two points are cited from: J.Farley and R. Gupta, PRA 15, 1952(1977)

Adiabatic Rapid Passage (ARP) Floquet theory [2] To get a large population transfer: Ω [2] J. H. Shirley, Phys. Rev. 138, B979(1965)

Population Transfer Time ( μs ) nm dye laser pulse Chirped microwave pulse Field ionization ramp 38d 36f

Conclusion Using microwave as a sensitive spectral probe, we measured the quantum defects of f 5/2,7/2 states. Using a chirped microwave pulse, we can transfer about 80% atoms from d states to f states.