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SrCl 2 crystal for EC/ + search Presented by J.H. So (KNU)
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Electron Capture/ + It is a kind of double + decay. + decay has three decay mode, such as EC/EC for less than 1 MeV Q-value, EC/ + for 1 MeV to 2 MeV Q-value, +/ + for more than 2 MeV Q-value. The Q-value of 84 Sr is 1.787 MeV, so EC/ + is possible.
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List of candidates NuclideDecay channel Q ββ, keV Natural abundance Decay modeLimits of Half-life (yr) 50 CrΕβ + 11714.3450v+2v1.8*10 17 58 NiΕβ + Εβ +,2E 192568.070v+2v 7*10 20 4.0*10 19 84 SrΕβ + 1786.80.560v7.3*10 13 96 Ru2β +,Eβ + 27195.540v+2v 3.1*10 16 6.7*10 16 106 Cd2β +, Eβ + 27711.250v+2v 0v 2.4*10 20 3.7*10 20 112 SnΕβ + 19220.970v6.1*10 13 124 Xe2β +,kβ + 28650.090v4.2*10 17 1.2*10 18 136 Ce2β +,kβ + 24000.1850v6.9*10 17 3.8*10 16 78 Kr2β +,kβ + 28660.350v+2v 0v 2*10 21 5.1*10 21 92 MoΕβ + Εβ +,2E 164914.840v+2v 1.9*10 20 3.0*10 18 EC/EC, EC/ +, +/ + had never been searched until today. We will search at 765 keV region for EC/ +.
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Test setup for SrCl 2 Pure SrCl 2 single crystal grown by CZ- method. (Jungin Kim) Cut and polished in the dimensions of 20 mm diameter and 15 mm height. Wrapped in teflon tape & mounted on 2 inch PMT with bialkali photocathode with the help of optical grease. Whole assembly is encased in a light tight covering. (details in Gulrooh’s talk) SrCl 2 PMT 400 MHz FADC High Voltage Computer SrCl 2 16.3 g (Sr 9 g)
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Relative light yield The light output of SrCl 2 single crystal is 77% of the light output of the CsI(Tl).
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Pulse height spectra of different radioisotopes
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Energy resolution Energy (keV) Resolution (FWHM) (%) 8114.8 8814.4 12215 51112.7 66210.5 83510.4 12757.6
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α/β α/β light ratio
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Fluorescence decay time Fast decay time component is 91 ns (12%) and slow decay time component is 907 ns(88%)
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Pulse shape discrimination Good discrimination between α- and γ-pulses, for pulse height corresponding to 1MeV energy range
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Experimental Technique Putting source(EC/ β + ) inside 4π CsI(Tl) crystals. Annihilation of β + gives the below possible signals. Using coincidence technique to tag the signals. Signal in figure 3 is the choice. Also we will use longitudinal back-to-back requirement with position measurement by attenuation length. No Yes Fig:1 Fig:2 Fig:3 511keV
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Schematic Preamp400MHz FADC 64MHz FADC ROOT High Voltage ☞ -670 V for SrCl 2 ☞ -1250 ~ -1450 V for 4 π CsI Threshold : 25 Trigger pulse width : 200 ns For SrCl 2 For 4 π CsI(Tl) 10 X 100 X
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Calibration ( 22 Na) We used 511 keV gamma ray for calibration and calculation of preliminary limit.
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Signals from SrCl 2 and 4 π CsI(Tl) + 3 days data
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SrCl 2 signals without 4 π CsI(Tl) signals 3 days data We want to search here.
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Expected SrCl 2 limits Q-value of 84 Sr is 1.7868 MeV & having natural abundance of 0.56%. The interesting energy is 765 keV with 511 keV back to back gamma coincidence. Preliminary limit : 1.84 X 10 18 years (Previous limit was 7.3 X 10 13 years.) This preliminary limit is calculated by CsI 0-hit data. After back to back coincidence analysis, it will be 10 times better than now. T 0n 1/2 = (ln2/1.64) 6x10 23 (a/A) (T/B R) at @ 90% C.L. B = background index in cts/(keV kg year) ⇒ 42,000 R = FWHM energy resolution at Q bb in keV ⇒ 16 % at 511 keV ( 22 Na) A = mass number ⇒ 87.62, e = detection efficiency at Q bb ⇒ 100% a = EC/ + isotope fraction ⇒ 0.05 g T = measured time in year ⇒ 1 year
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Pure SrCl 2 single crystal developed for the first time of the neutrinoless EC/β + search. The scintillation properties of SrCl 2 was good for EC/ + search. The preliminary limit is 1.84 X 10 18 years. (Previous limit was 7.3 X 10 13 years.) We will take data for 3 months. Further background reduction is expected with triple coincidence between + signal and back to back coincidence. We will investigate the contamination of 90 Sr.( decay Q value = 2.27 MeV) from nucleon fall out. Summary and Future plan
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