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YAK-Aerosib : Study on tropospheric composition over Siberia
Jean-Daniel Paris1 Ph. Nedelec2, M. Ramonet1, G. Golytsin3, B. Belan4, M. Arshinov4, G. Athier2, F. Boumard1, J.-M. Cousin2 , et Ph. Ciais1 Thanks Robert Vautard [LSCE] MM5-Chimere Gregoire Cayez [Lab. d’Aérologie] & Andreas Stohl [NILU, Norvège] Flexpart Frederic Chevallier [LSCE] données ECMWF Joyce Harris [NOAA, USA] clusters Hysplit 1 Laboratoire des Sciences du Climat et de l'Environnement IPSL, CEA-CNRS-UVSQ, Saclay 2 Laboratoire d’Aérologie UPS-CNRS, Toulouse 3 Institute of Atmospheric Physics RAS, Moscow, Russia 4 Institute of Atmospheric Optics SB-RAS, Tomsk, Russia
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YAK-Aerosib, J.-D. Paris et al.
Background & Goals Background : Siberia represents 32% of global soil carbon pool. Sink estimated 0.0 – 1.0 GtC.yr-1 (Gurney, Nature, 2002) Extratropical Asia is scarcely touched by studies on atmospheric transport in the Northern hemisphere (Akimoto, Science, 2003) Goals : Bring new constraints on Siberian CO2 sources and sinks Characterize the variability of ozone and CO at the continental scale. YAK-Aerosib, J.-D. Paris et al.
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YAK-Aerosib, J.-D. Paris et al.
Antonov-30 platform Flight ceiling – 8100 m Flight duration – 8 hr Endurance – 3400 km Max flight speed – 540 km/h Speed during measurements – 300 km/h Runway length – 1300 m Aircraft crew – 7 pilots Science crew – <10 persons Aircraft length – 24.3 m Aircraft height – 8.3 m YAK-Aerosib, J.-D. Paris et al.
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Intensive airborne campaigns first measurements
1. Intensive airborne campaigns first measurements YAK.1/11-14 April 2006 YAK.2/7-10 September 2006 Profiles CO2, CO & O3
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Instrumental Setup CO2 CO + O3 Antonov 30 Methane CO2 13C isotope
CURRENTLY OPERATED CO2 LSCE, Saclay. In operation CO + O3 LA, Toulouse. In operation Antonov 30 IAO, Tomsk (shown: Inlet) TO BE DEPLOYED Methane LSP, Grenoble. Test phase CO2 13C isotope LPMAA, Paris. Test phase Flask sampler MPI-BGC, Jena. Ready YAK-Aerosib, J.-D. Paris et al.
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Flight pattern 3 days of flight 2-8 vertical legs per flight from 500 to 7000 m agl 8000km across Siberia 7km YAK-Aerosib, J.-D. Paris et al.
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Meteorological conditions, april
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Meteorological conditions, sept.
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Average profiles YAK-Aerosib, J.-D. Paris et al.
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mozaic Data: Valérie Thouret, L.A., pers. comm. spring summer Fall winter YAK-Aerosib, J.-D. Paris et al.
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Pollutants transport in Siberia
2. Pollutants transport in Siberia
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Anthropic emissions origines during the campaigns
Flexpart (ECMWF fields) YAK-Aerosib, J.-D. Paris et al.
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Polluted layers detection
Stratification, polluted filaments over 500km in the horizontal 60°N-120°E 3nm<dp<70nm dp>70nm Aerosol number conc, cm-3 YAK-Aerosib, J.-D. Paris et al.
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April: N-E China affect [CO] over Siberia
YAK1& Mopitt 173 ppb 190 ppb YAK1: 4-6km, flight segment average & MOPITT April average at 500hPa YAK-Aerosib, J.-D. Paris et al.
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From China to Siberia Flexpart: retroplume 10 days back Interception of a polluted dust storm 2002 MODIS/Terra YAK-Aerosib, J.-D. Paris et al.
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Chemistry transport eulerian study
Regional CTM: MM5-Chimere 1.0 x 0.75°, 10 levels [CO] (anomaly from N-E China emissions) defined as: (reference run) minus (run with all but NE Chinese emissions) YAK trajectory shown 2006/04/12, 0400GMT z ~ m YAK-Aerosib, J.-D. Paris et al.
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Chinese pollutant export : episode toward Sibérie and Taiwan
DCO Hovmöller diagram of the event simulation MM5-Chimere YAK-Aerosib, J.-D. Paris et al.
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OMI Aerosol index YAK-Aerosib, J.-D. Paris et al.
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WCB frequency to East Siberia
3-yr Climatology of air masses monthly origin: September Hysplit backtrajectories cluster analysis, september (Joyce Harris, NOAA) YAK-Aerosib, J.-D. Paris et al.
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3. CO2 variability
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CO2 – CO correlation YAK-Aerosib, J.-D. Paris et al.
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7 September 2006 as an example
Zonal flux, crossing a weak front High variability between consecutive CO2 profiles YAK-Aerosib, J.-D. Paris et al.
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CO2 Boundary layer variogram
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Conclusion & Perspectives
Presentation of YAK campaigns and data Continental variability of CO2 during growth season strongly affected by synoptic conditions Pollutants transport des in Siberia: chinese episode, european transport Evolving: Using MM5-Chimère to quantify flux of pollutants toward Siberia (climatology, event-based) Characterization of transport for the study of CO2 fluxes, lagrangian model, CO surrogate tracer Inversion (LPDM?) to better constrain CO2 sources and sinks Contribution to Polarcat Provide an (almost) “off the shelf” campaign in Siberia equipped with instruments for CO2, CO, ozone, aerosols number conc., … Advantage: blank spot in observation networks Limitations: new instruments? Difficulty to change flight route? YAK-Aerosib, J.-D. Paris et al.
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