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Photodetachment microscopy to an excited state and accurate electron affinity measurements
C. Blondel, C. Delsart, C. Drag, R. J. Peláez & M. Vandevraye Laboratoire Aimé-Cotton, bât. 505, CNRS, université Paris-sud, F Orsay cedex, France Photodetachment microscopy Photodetachment microscopy to an excited state: 31P- hν a Level scheme Classical parameters Highest height Maximum radius z0 = Quantum parameters : Wavelength scale Number of rings Interfrange distance Radial current density 0 = m a = 0.35 m R F = 427 Vm-1 = 0,926 ± 0,002 cm-1 Rmax j Principle: Y.N. Demkov et al., JETP Lett. 34 (1981) 403 Photodetachment microscopy: C. Blondel et al., Phys. Rev . Lett. 77 (1996) 3755 Photoionization microscopy: C. Nicole et al., Phys. Rev . Lett. 88 (2002) Molecular photodetachment microscopy : C. Delsart et al., Phys. Rev . Lett. 89 (2002) Linear regression to zero kinetic energy Experimental set-up Measured thresholds Experimental spots Deduced intervals C D F U negative ion neutral atom h eA Electron affinity (10), formerly (6) eV Neutral atom spectroscopy and fine structure 15 7 6 5 4 3 2 1 8 9 10 11 12 13 Photodetachment microscopy of Se- 14 Electron affinity : (8) m-1 formerly (20) m-1 or (1) vs (2) eV 4 : Wien filter 7 : Deflection 11 : Focalisation quadrupole 12 : Deceleration plates 13 : Interaction zone 14 : Laser 15 : Column of constant F 16 : MCP 17 : Phosphor screen 18 : CCD 1 : Source and simple lens doublet (“Einzellens") 2,5,9,10 : Deflection plates 3,6,8 : Simple lenses 43rd EGAS, Fribourg, 28 June – 2 July 2011
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