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Published byHedvig Toft Modified over 6 years ago
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EMIS: Improve Emission Inventories of Environmentally Relevant Species
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Agenda 11:00 Introduction – Randall Martin
11:10 ICARTT briefing – Daniel Jacob 11:25 Emission inventory assessment – David Parrish 11:40 Bottom-up inventory development – Ted Russell 12:00 lunch 1:30 NRT SCIAMACHY retrievals – Andreas Heckel 1:45 SAO retrievals – Kelly Chance 2:00 Preliminary SCIAMACHY/in situ comparison – Chris Sioris 2:15 VOC emissions – Paul Palmer 2:30 Action items – Randall Martin 2:40 Discussion 4 Adjourn
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Weight by relative uncertainty
What Is Needed To Use Satellite Observations to Improve Emission Inventories? Top-down emissions & uncertainty Include in model Optimized inventory & uncertainty Test with correlative in situ obs Weight by relative uncertainty Bottom-up emissions & uncertainty O3, NO, NO2, PAN, HNO3, HCHO, … Quantified uncertainty in top-down inventory Quantified uncertainty in bottom-up inventory Ideally, attribution of differences to source type
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Calculate Top-Down NOx Emissions from GOME/SCIAMACHY/OMI SCIAMACHY Tropospheric NO2
May 2004 Short NOx lifetime and dominance of NO2 near surface simplify calculation (top-down NOx emissions) Et = t (satellite NO2 column observation) Calculate locally with model as Ea/a (iterate if nonlinear) Quantify uncertainty in satellite obs (validation and error propagation) Quantify uncertainty in model chemistry (and transport)
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How Can Different Source Types Be Isolated
How Can Different Source Types Be Isolated? By Day of the Week Variation Friday Saturday Sunday 1015molec/cm2 Beirle et al., ACP, 2003
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How Can Different Source Types Be Isolated
How Can Different Source Types Be Isolated? By Residual: Soils Contribute 40% of Surface NOx Emissions from Africa Jaeglé, Martin, et al., JGR, in press
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