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Magnetic field induced charge-density-wave transitions: the role of orbital and Pauli effects
Mark Kartsovnik Walther-Meißner-Institut, BADW, Garching, Germany
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Outline
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a-(BEDT-TTF)2KHg(SCN)4: basic features
r||(300 K) 30 – 100 Wcm; r^/r|| ~ ; r||(300 K)/ r||(1.4 K) 102 T. Mori et al., 1990 2D Fermi surface Nesting instability of the Fermi surface CDW formation at 8 K very low!! Q
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Pauli effect (isotropic)
Spin splitting deteriorates the nesting conditions for a CDW TCDW/TCDW(0), exp Phase diagram of a-(BEDT-TTF)2KHg(SCN)4 P. Christ et al., JETP Lett. 2000 ~ 23 T Q+ Q- TCDW/TCDW(0) Theory: D. Zanchi et al., PRB 1996; P. Grigoriev&D.Lyubshin , PRB 2005 B suppresses CDW Q- < Q+
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Orbital effect (B || z) Dy ~ 1/Bz Real space orbit: electrons become
effectively more 1D Real space orbit:
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Orbital effect (B || z) FICDW at t^’ > t^’ * Theory
a-(BEDT-TTF)2KHg(SCN)4 D. Andres et al., PRB 2001 Theory FICDW at t^’ > t^’ * due to Landau quantization of the unnested FS pocket D. Zanchi et al., PRB 1996
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FICDW: experiment; B || z
SdHo The “slow oscillations” approximately periodic with 1/B appear at P Pc 2.5 kbar display a weak hysteresis P = 3 kbar
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FICDW: experiment; B || z
The “slow oscillations” approximately periodic with 1/B appear at P Pc 2.5 kbar display weak hysteresis slightly shift with temperature behaviour consistent with the FICDW scenario!!
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FICDW: experiment; B || z
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FICDW: experiment; B || z
in a-(BEDT-TTF)2KHg(SCN)4 FISDW in (TMTSF)2PF6 A. Kornilov et al., PRB 2002 FICDW is weaker than FISDW due to the Pauli effect! A. Lebed, JETP Lett. 2003
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FICDW: role of the Pauli effect
N = 5 4 3 2 1 4 N = 3 2 1 no Pauli effect (FISDW) Pauli effect on (FICDW) Qx = 2kF + NG Qx = 2kF QP + NG G = 2eayBz/h QP = 2mBB/hvF
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FICDW: role of the Pauli effect
4 N = 3 2 1 A. Lebed, JETP Lett. 2003 no Pauli effect (FISDW) Pauli effect on (FICDW) Qx = 2kF + NG Qx = 2kF QP + NG G = 2eayBz/h QP = 2mBB/hvF
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FICDW in a tilted field Commensurate splitting “Spin-zero” 2QP = MG
(A. Bjelis et al., 1999; A. Lebed, 2003) “Spin-zero” N = 3,4 2,3 1,2 0,1 2QP = MG 2QP = (M + 1/2)G with M - integer A. Lebed, JETP Lett. 2003
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FICDW in a tilted field: experiment
T = 0.4 K Spin-zero condition:
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FICDW in a tilted field: experiment
1st CS angle Spin-zero condition:
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FICDW in a tilted field: experiment
1st CS angle Spin-zero condition: vF 1.2105 m/s
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Summary The orbital effect causes FICDW transitions in a-(BEDT-TTF)2KHg(SCN)4 at pressures above Pc = 2.5 kbar The Pauli effect, in general, weakens the FICDW instability The interplay between the orbital and Pauli effects can be controlled by changing the field orientation: - the FICDW is enhanced at commensurate splitting angles - the FICDW is suppressed at „spin-zero“ angles
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