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Perovskite nanowire–block copolymer supramolecular nanocomposites

Published byClemens Bachmeier Modified over 5 years ago

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Presentation on theme: "Perovskite nanowire–block copolymer supramolecular nanocomposites"— Presentation transcript:

1 Fig. 1 Perovskite nanowire–block copolymer supramolecular nanocomposites.
Perovskite nanowire–block copolymer supramolecular nanocomposites. (A) Schematic diagram of the perovskite crystal structure. (B) PL of CsPbX3 (X = I, Br, and Cl) perovskite nanowires in toluene solution. Halide composition determines the material’s bandgap and color of emitted light (λexcitation = 380 nm). (C) TEM images of naturally aligned bundles of CsPbBr3 perovskite nanowires (length, ~1 μm; diameter, ~10 nm). (D) TEM images (top) and SAXS measurements (bottom) of the pure SIS filaments without nanowires printed using 1-mm-diameter nozzle (left, horizontally printed sample; right, filament cross sections), demonstrating microphase separated SIS hexagonal domains with long-range order and anisotropy. Red arrow indicates printing and the microdomain alignment direction. (E) A maximum intensity projection of z-stack fluorescence confocal image of the printed nanowire-block copolymer filament (diameter, 100 μm; λexcitation = 365 nm). (F) Representative TEM images of nanocomposite filaments printed using 1-mm-diameter nozzle showing perovskite nanowires oriented in parallel with the print direction and locally conform to the SIS block copolymer microdomains. A higher-magnification TEM image (inset) shows that nanowires primarily segregate to PI-rich domains (see also fig. S6 and table S4). The TEM samples in (D) and (F) are sectioned using cryo-ultramicrotome and stained with OsO4, which selectively darkens the PI domains. Nanjia Zhou et al. Sci Adv 2019;5:eaav8141 Copyright © 2019 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC).

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