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Sliding of a charge density wave probed by coherent X-Ray Diffraction E. Pinsolle Laboratoire de physique des solides, Orsay
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Synchrotron Sources Experiment caried out by: E. Pinsolle V. Jacques D. Le bolloc’h A. Sinchenko P. Monceau Experiment done at the ESRF on the beamline ID10A
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NbSe3 sample Sample dimensions: 2mm x 10μm x 10μm 3 types of chains: -first one with Peierls transition at 145K -second one with Peierls transition at 59K -last one with no transition. Threshold current 0.9 mA
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Signature of CDW in X-ray diffraction Gap opening at the fermi level. Electron density modulation -2k F +2k F Spawning of satellites around initial Bragg peak. Satellite reflection (0 1.25 0)
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Experimental setup Incident X ray beam Chain axis Diffracted Beam CCD camera Gold contacts Two interest of this experiment: -Coherent beam sensitive to phase defects. -Micrometer scale beam.
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Above the threshold Bellow the threshold 2D diffraction patterns Increasing current values I=0 mA I=0.8 mA I=1.4 mA I=1.8 mA I=0.2 mA I=0.4 mA I=0.6 mA I=1.6 mA
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First Result: Satellite in transverse direction. Satellite in the transverse direction for different current value, bellow (colon 1) and above (colon 2) the threshold. (I S =0.9 mA) Satellite with I=1.8 mA Satellite with I=0.2 mA
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The shift of the satellite change sign when we exceed the threshold. -No speckle and no shape change. The shift δq= +/- 0.26 10 -4 Å -1 which correspond in the real space to a change of the wave length δλ=+/- 8.10 -4 Å Second Result: Satellite in longitudinal direction. Satellite in direction of chain axis for different current value, under (colon 1) and above (colon 2) the threshold. (I S =0.9 mA)
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Speckle signature of creep Bellow threshold Phase equation: -We suppose to be in a stationary case. - Correlations in longitudinal direction are much higher than in transverse direction. This lead to the following phase equation:
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Influence of steps above threshold Chain axis The CDW must vanish at the interface of the step. Nb Se3 is known to have step at the surface
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If some strong pinning defects are present on chain d n, this fixe the phase on these chain (φ(d n )=0) and leads to the solution: simulation from the previous theory compared to experiment. dndn d n-2 d n-1 φnφn Φ n-1 0 φ Speckle signature of creep Bellow threshold
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2k F contraction Bellow the threshold. Theoretical explanation: where The total number of carriers is conserved. But when some current is applied we create a disequilibrium of the normal carrier densities. Approximate view of the band structure δqδq
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Current conversion above the threshold. Stress experienced by the CDW Chain axis Gold contacts δλδλ δqδq δλ=0 P. Monceau et al. Plastic sliding of charge density waves. Physical review B
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Conclusion Thank you for your attention! Different behaviors of the CDW under current probed by coherent X ray diffraction: Bellow the threshold: Along the transverse direction. We observe phase defects which is the signature of creep phenomenon. Along longitudinal direction. Condensation of normal electrons in the CDW. Above the threshold: Along transverse direction. Influence of steps on the CDW. Along longitudinal direction. Current conversion far from contacts.
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