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M. Hücker Manipulating Competing Order with High Pressure Neutron Scattering Group (CMPMS) Correlated Electron Systems ( Superconductivity, Magnetism,

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Presentation on theme: "M. Hücker Manipulating Competing Order with High Pressure Neutron Scattering Group (CMPMS) Correlated Electron Systems ( Superconductivity, Magnetism,"— Presentation transcript:

1 M. Hücker Manipulating Competing Order with High Pressure Neutron Scattering Group (CMPMS) Correlated Electron Systems ( Superconductivity, Magnetism, Electronic Order)  High Temperature Superconductors  Transition Metal Oxides  Ferroelectrics  Heavy Fermion Systems  Multiferroics La 2-x Ba x CuO 4 Charge & Spin Stripes

2 LBCO CGO 1 mm Single-Crystal XRD at Low Temperature 360° X-ray window  Intensity ~10 -6 off strongest Bragg Peak  Powder XRD not possible  E=100keV, 210 11 photons/sec/mm 2 BW5-HASYLAB

3 High Pressure Beamline at NSLS-II  Single Crystal XRD  4-Circle Diffractometer  Point Detector (2D Detector optional)  Low Temperature  Flux >10 11 –10 12 photons/sec on Sample  DAC (MAC,Toroid)  Sample Centering  M. v. Zimmermann, HASYLAB  J. M. Tranquada, G. Xu, Neutron Scattering Group  Y. J. Kim, University of Toronto  B. Wells, University of Connecticut  D. J. Buttrey, University of Delaware  C. C. Kao, Z. Zhong, NSLS

4 NSLS II Paris Edinburgh Cell 100 mm 3 30 GPa 25 kg low T not so easy Diamond Anvil Cell 0.0001 mm 3 100 GPa small beam sample position pressure inhomogeneous ISIS

5 Yamada et al. JSSC 1989 Bozovic et al. PRL 2002 LSCO thin film LSCO bulk Gao et al. PRB 1994 Hg-1223 bulk Pressure and Superconductivity Pressure: affects crystal structure and electronic band structure buckled flat

6 Competing order in LBCO single-crystal HXRD

7 Charge Stripes under Pressure LTT structure Charge Stripes Do stripes survive in flat planes when x=1/8?

8 Hole Crystallization in 2-Leg Ladder Blumberg et al. Science 2002 Rusydi et al. Sr 14 Cu 24 O 41 Abbamonte et al. RSXS oxygen-K edge XRD: Zimmermann et al. PRB 2006

9 3 GPa 4 GPa 7 GPa NSLS/HASYLAB/NSLSII 100keV Large Volume Pressure Cells for Single-Crystal X-ray Diffraction 100keV Mini Toroid Cell 1 cm

10 pressure cell: scattering/absorption pressure cell absorption: factor 10

11 pressure sensor: CuGeO 3 structural distortion at the spin Peierls transition at 14 K

12 100 keV beamline BW5 at HASYLAB, Hamburg E-range: 60-200 keV Crystal type: Si/TaSi 2 (100”) Si 1-x Ge x (15”–70”) Our Exp: 35” E-resolution: 600eV at 100keV Flux(photons/s): 2e11/mm 2 @ 100keV (100mA, 4.5GeV) Spot size: 0.5mm x 0.5mm to 6mm x 6mm Detector: N 2 cooled Ge det. Wiggler: 2Tesla, 17 periods

13 Competing Order Lattice density (pressure) Charge density (doping) CePd 2 Si 2


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