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CH3Br, 101209 1)“New” C atomic lines 2)Summary of C atomic line observations and “nonobservations” agust,heima,....Dec09/CH3BR-Overall (C)-081209km agust,www,...Dec09/PPT-101209aak.ppt.

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Presentation on theme: "CH3Br, 101209 1)“New” C atomic lines 2)Summary of C atomic line observations and “nonobservations” agust,heima,....Dec09/CH3BR-Overall (C)-081209km agust,www,...Dec09/PPT-101209aak.ppt."— Presentation transcript:

1 CH3Br, 101209 1)“New” C atomic lines 2)Summary of C atomic line observations and “nonobservations” agust,heima,....Dec09/CH3BR-Overall (C)-081209km agust,www,...Dec09/PPT-101209aak.ppt agust,heima,...Dec09/XLS-101209ak.xls

2 New 3 peaks New ?? artifact ATH?

3 71343.2474 71349.2 71353.3

4 Configuration Term J Level (cm -1 ) 2s22p2 2s22p2 3 P 0 0 1 16.40 2 43.40 2s22p2 2s22p2 1 D 2 10 192.63 2s22p2 2s22p2 1 S 0 21 648.01 2s2p3 2s2p3 5 S° 2 33 735.20 2s 2 2p( 2 P°)3s 3 P° 0 60 333.43 1 60 352.63 2 60 393.14 2s 2 2p( 2 P°)3s 1 P° 1 61 981.82 2s2p3 2s2p3 3 D° 3 64 086.92 1 64 089.85 2 64 090.95 2s 2 2p( 2 P°)3p 1 P 1 68 856.33 2s 2 2p( 2 P°)3p 3 D 1 69 689.48 2 69 710.66 3 69 744.03 2s 2 2p( 2 P°)3p 3 S 1 70 743.95 2s 2 2p( 2 P°)3p 3 P 0 71 352.51 1 71 364.90 2 71 385.38 2s 2 2p( 2 P°)3p 1 D 2 72 610.72 2s 2 2p( 2 P°)3p 1 S 0 73 975.91 J GS0 0 3P116.4 243.4 2s22p(2Po)3p071352.5171336.1171309.11 3P171364.971348.571321.5 271385.3871368.9871341.98 agust,heima,...Dec09/XLS-101209ak.xls: http://physics.nist.gov/cgi-bin/ASD/energy1.plhttp://physics.nist.gov/cgi-bin/ASD/energy1.pl :

5 Check 69704.95668/ 69705.0 To be copaierd with lines in PPT-240809ak.ppt:

6 Configurati on Term J Level (cm -1 ) 2s22p2 2s22p2 3 P 0 0 1 16.40 2 43.40 2s22p2 2s22p2 1 D 2 10 192.63 2s22p2 2s22p2 1 S 0 21 648.01 2s2p3 2s2p3 5 S° 2 33 735.20 2s 2 2p( 2 P°)3 s 3 P° 0 60 333.43 1 60 352.63 2 60 393.14 2s 2 2p( 2 P°)3 s 1 P° 1 61 981.82 2s2p3 2s2p3 3 D° 3 64 086.92 1 64 089.85 2 64 090.95 2s 2 2p( 2 P°)3 p 1 P 1 68 856.33 2s 2 2p( 2 P°)3 p 3 D 1 69 689.48 2 69 710.66 3 69 744.03 2s 2 2p( 2 P°)3 p 3 S 1 70 743.95 2s 2 2p( 2 P°)3 p 3 P 0 71 352.51 1 71 364.90 2 71 385.38 C I69647.2 69668.9 69675.3 69697.7 69705.0 69715.4 69733.1 1D REMPI for C + Measurements seem to have got lost http://physics.nist.gov/cgi-bin/ASD/energy1.pl Exp. Values:

7 71343.2474~71341.98 J’’=2 ->-> J´=2 71349.2 ~71348.5; J’’= 1 ->-> J´= 1 71353.3 ~ 71352.51; J’’=0 ->-> J´=0 Ergo: The lines are: 2s22p2 (3P) ->-> 2s22p(2P°)3p(3P),  J =0:

8 77411.21 Does not seem to be C atomic line. (see: agust,heima,...Dec09/XLS-101209ak.xls ) Could this be Br atomic line?...... NO, not according to....PPT-201009aak.ppt

9 Now lets check C atomic lines for 2p 2 ->-> np transitions 1) 3 P ->> 3 X 2) 1 D ->-> 1 X :

10 Configuration Term J Level (cm -1 ) 2s22p2 2s22p2 3 P 0 0 1 16.40 2 43.40 2s22p2 2s22p2 1 D 2 10 192.63 2s22p2 2s22p2 1 S 0 21 648.01 2s2p3 2s2p3 5 S° 2 33 735.20 2s 2 2p( 2 P°)3s 3 P° 0 60 333.43 1 60 352.63 2 60 393.14 2s 2 2p( 2 P°)3s 1 P° 1 61 981.82 2s2p3 2s2p3 3 D° 3 64 086.92 1 64 089.85 2 64 090.95 2s 2 2p( 2 P°)3p 1 P 1 68 856.33 2s 2 2p( 2 P°)3p 3 D 1 69 689.48 2 69 710.66 3 69 744.03 2s 2 2p( 2 P°)3p 3 S 1 70 743.95 2s 2 2p( 2 P°)3p 3 P 0 71 352.51 1 71 364.90 2 71 385.38 2s 2 2p( 2 P°)3p 1 D 2 72 610.72 2s 2 2p( 2 P°)3p 1 S 0 73 975.91 2s2p3 2s2p3 3 P° 1 75 253.97 2 75 255.27 0 75 256.12 2s 2 2p( 2 P°)3d 1 D° 2 77 679.82 2s 2 2p( 2 P°)4s 3 P° 0 78 104.98 1 78 116.74 2 78 148.09 2s 2 2p( 2 P°)3d 3 F° 2 78 199.07 3 78 215.51 4 78 249.94 2s 2 2p( 2 P°)3d 3 D° 1 78 293.49 2 78 307.63 3 78 318.25 2s 2 2p( 2 P°)4s 1 P° 1 78 340.28 2s 2 2p( 2 P°)3d 1 F° 3 78 529.62 2s 2 2p( 2 P°)3d 1 P° 1 78 731.27 2s 2 2p( 2 P°)3d 3 P° 2 79 310.85 1 79 318.78 0 79 323.16 2s 2 2p( 2 P°)4p 1 P 1 80 562.85 2s 2 2p( 2 P°)4p 3 D 1 80 782.51 2 80 801.27 3 80 834.61 Observed New (101209) Not observed observed Not observed(?) Not observed limit

11 2s 2 2p( 2 P°)4p 3 S 1 81 105.03 2s 2 2p( 2 P°)4p 3 P 0 81 311.01 1 81 325.76 2 81 343.99 2s 2 2p( 2 P°)4p 1 D 2 81 769.79 2s 2 2p( 2 P°)4p 1 S 0 82 251.71 2s 2 2p( 2 P°)4d 1 D° 2 83 497.62 2s 2 2p( 2 P°)5s 3 P° 0 83 740.06 1 83 752.41 2 83 791.04 2s 2 2p( 2 P°)4d 3 F° 2 83 747.39 3 83 761.26 4 83 798.57 2s 2 2p( 2 P°)4d 3 D° 1 83 820.13 2 83 838.08 3 83 848.83 2s 2 2p( 2 P°)5s 1 P° 1 83 877.31 2s 2 2p( 2 P° 1/2 )4f 2 [ 5 / 2 ] 3 83 919.65 2 83 919.76 2s 2 2p( 2 P° 1/2 )4f 2 [ 7 / 2 ] 3 83 926.20 4 83 926.37 2s 2 2p( 2 P°)4d 1 F° 3 83 947.43 2s 2 2p( 2 P° 3/2 )4f 2 [ 7 / 2 ] 3 83 986.22 4 83 986.45 2s 2 2p( 2 P° 3/2 )4f 2 [ 5 / 2 ] 3 84 013.25 2 84 013.40 2s 2 2p( 2 P° 3/2 )4f 2 [ 9 / 2 ] 5 84 015.86 4 84 016.25 2s 2 2p( 2 P°)4d 1 P° 1 84 032.15 2s 2 2p( 2 P° 3/2 )4f 2 [ 3 / 2 ] 1 84 036.29 2 84 036.40 2s 2 2p( 2 P°)4d 3 P° 2 84 103.10 1 84 116.09 0 84 121.22 2s 2 2p( 2 P°)5p 1 P 1 84 851.53 2s 2 2p( 2 P°)5p 3 D 1 84 935.34 2 84 950.36 3 84 984.97 2s 2 2p( 2 P°)5p 3 P 0 85 169.61 1 85 188.95 2 85 203.64 2s 2 2p( 2 P°)5p 1 D 2 85 399.81 2s 2 2p( 2 P°)5p 1 S 0 85 625.18 2s 2 2p( 2 P°)5d 1 D° 2 86 185.20 2s 2 2p( 2 P°)5d 3 F° 2 86 317.64 3 86 327.16 4 86 369.47 2s 2 2p( 2 P°)6s 3 P° 0 86 321.94 1 86 331.63 2 86 369.60 2s 2 2p( 2 P°)5d 3 D° 1 86 362.52 2 86 389.38 3 86 397.80 2s 2 2p( 2 P°)6s 1 P° 1 86 416.55 2s 2 2p( 2 P°)5d 1 F° 3 86 449.19 Not observed observed Weak but Observable See below 1)

12 2s 2 2p( 2 P° 3/2 )5f 2 [ 7 / 2 ] 3 86 469.51 4 86 469.66 2s 2 2p( 2 P° 3/2 )5f 2 [ 5 / 2 ] 3 86 482.66 2 86 482.78 2s 2 2p( 2 P°)5d 1 P° 1 86 491.41 2s 2 2p( 2 P° 3/2 )5f 2 [ 3 / 2 ] 1 86 498.55 2 86 498.64 2s 2 2p( 2 P°)5d 3 P° 2 86 506.70 1 86 519.47 0 86 523.16 2s 2 2p( 2 P°)6p 1 P 1 86 912.86 2s 2 2p( 2 P°)6p 3 D 1 86 956.16 2 86 965.45 3 87 002.26 2s 2 2p( 2 P°)6p 3 P 0 87 077.36 1 87 103.12 2 87 113.21 2s 2 2p( 2 P°)6p 1 D 2 87 218.26 2s 2 2p( 2 P°)6p 1 S 0 87 341.04 2s 2 2p( 2 P°)6d 1 D° 2 87 633.75 2s 2 2p( 2 P°)6d 3 F° 2 87 708.21 3 87 713.38 4 87 760.61 2s 2 2p( 2 P°)7s 3 P° 0 87 711.37 1 87 718.56 2 87 753.73 2s 2 2p( 2 P°)6d 3 D° 1 87 735.30 2 87 773.09 3 87 777.17 2s 2 2p( 2 P° 1/2 )6f 2 [ 7 / 2 ] 4 87 763.10 3 87 763.24 2s 2 2p( 2 P°)7s 1 P° 1 87 789.63 2s 2 2p( 2 P°)6d 1 F° 3 87 806.93 2s 2 2p( 2 P° 3/2 )6f 2 [ 5 / 2 ] 3 87 826.94 2 87 827.02 2s 2 2p( 2 P°)6d 1 P° 1 87 830.17 2s 2 2p( 2 P°)6d 3 P° 2 87 832.54 1 87 843.91 0 [87 846.9] [] 2s 2 2p( 2 P° 3/2 )6f 2 [ 3 / 2 ] 1 87 837.74 2 2s 2 2p( 2 P°)7p 1 P 1 88 061.28 2s 2 2p( 2 P°)7p 3 D 1 88 092.01 2 88 096.03 3 88 135.81 2s 2 2p( 2 P°)7p 3 P 0 88 159.87 1 88 192.30 2 88 198.22 2s 2 2p( 2 P°)7p 1 D 2 88 260.37 2s 2 2p( 2 P°)7p 1 S 0 88 333.98 2s 2 2p( 2 P°)7d 1 D° 2 88 498.62 Not observed observed Not observed

13 2s 2 2p( 2 P°)7d 3 F° 2 [88 541.4] [] 3 [88 544.9] [] 4 [88 596.5] [] 2s 2 2p( 2 P°)8s 3 P° 0 88 543.76 1 88 549.06 2 88 584.26 2s 2 2p( 2 P°)7d 3 D° 1 [88 558.6] [] 2 88 604.75 3 [88 606.8] [] 2s 2 2p( 2 P° 1/2 )7f 2 [ 5 / 2 ] 2 88 574.85 2s 2 2p( 2 P°)8s 1 P° 1 88 615.01 2s 2 2p( 2 P°)7d 1 F° 3 88 625.00 2s 2 2p( 2 P° 3/2 )7f 2 [ 7 / 2 ] 3 88 633.98 4 88 634.07 2s 2 2p( 2 P°)7d 3 P° 2 [88 636.8] [] 1 [88 646.6] [] 0 [88 649.1] [] 2s 2 2p( 2 P° 3/2 )7f 2 [ 5 / 2 ] 3 88 638.30 2s 2 2p( 2 P°)7d 1 P° 1 88 639.02 2s 2 2p( 2 P° 3/2 )7f 2 [ 3 / 2 ] 2 88 645.33 2s 2 2p( 2 P°)8p 1 P 1 88 766.98 2s 2 2p( 2 P°)8p 3 D 1 88 790.85 2 [88 794.3] [] 3 88 836.12 2s 2 2p( 2 P°)8p 3 P 2 88 873.95 2s 2 2p( 2 P°)8p 1 D 2 88 913.56 2s 2 2p( 2 P°)8p 1 S 0 88 960.64 2s 2 2p( 2 P°)8d 1 D° 2 89 054.16 2s 2 2p( 2 P°)8d 3 F° 2 [89 079.9] [] 3 [89 082.1] [] 4 [89 136.9] [] 2s 2 2p( 2 P°)9s 3 P° 0 89 081.62 1 89 085.41 2s 2 2p( 2 P°)8d 3 D° 1 [89 091.8] [] 2 89 142.66 3 [89 143.4] [] 2s 2 2p( 2 P° 1/2 )8f 2 [ 5 / 2 ] 2 89 101.76 3 89 101.79 2s 2 2p( 2 P°)9s 1 P° 1 89 149.35 2s 2 2p( 2 P°)8d 1 F° 3 89 155.70 2s 2 2p( 2 P° 3/2 )8f 2 [ 7 / 2 ] 4 89 162.10 2s 2 2p( 2 P°)8d 3 P° 0 [89 171.5] [] 1 [89 170.0] [] 2 [89 162.2] [] 2s 2 2p( 2 P°)8d 1 P° 1 89 164.74 2s 2 2p( 2 P°)9p 1 P 1 89 232.41 2s 2 2p( 2 P°)9p 3 D 3 89 299.10 2s 2 2p( 2 P°)9p 1 D 2 89 350.10 2s 2 2p( 2 P°)9p 1 S 0 89 381.61 : Not observed 91193:limit

14 71577.6(obs.) vs 71577.16 (predicted) 72061.4 (obs.) vs 72059.1 (predicted) 1)

15 Agust,heima,...Dec09/AFSTODUMYND-190809hrh-101209ak.pxp

16 69689.48/2 3 P-> 3 D J´´=0 ->>J´=1 H 2 + C( 3 P) +HBr 59329 69689.48/2 3 P-> 3 D J’´=0 ->>J´=1 10360.48 H 2 + C*( 1 D) +HBr 69521.63 H 2 + C**( 3 D) +HBr H 2 + C**( 3 P) +HBr (H 2 + C**(4p, 1 D) +HBr) (H 2 + C**(4p, 1 S) +HBr) H 2 + C**(5p, 1 D) +HBr H 2 + C**(5p, 1 S) +HBr H 2 + C**(6p, 1 D) +HBr H 2 + C**(6p, 1 S) +HBragust,heima,...Dec09/AFSTODUMYND-190809hrh-101209ak.pxp

17 71352.51/2 3 P-> 3 P J’´=0 ->>J´=0 H 2 + C +HBr 59329 71352.51/2 3 P-> 3 P J’´=0 ->>J´=0 H 2 + C*(1D) +HBr 69521.63 12023.51 H 2 + C**( 3 D) +HBr H 2 + C**( 3 P) +HBr (H 2 + C**(4p, 1 D) +HBr) (H 2 + C**(4p, 1 S) +HBr) H 2 + C**(5p, 1 D) +HBr H 2 + C**(5p, 1 S) +HBr H 2 + C**(6p, 1 D) +HBr H 2 + C**(6p, 1 S) +HBragust,heima,...Dec09/AFSTODUMYND-190809hrh-101209ak.pxp

18 71577.16/2 1 D->->4p, 1 D H 2 + C +HBr 59329 H 2 + C*( 1 D) +HBr 69521.63 71577.16/2 1 D->->4p, 1 D Very week 2055.52 H 2 + C**( 3 D) +HBr H 2 + C**( 3 P) +HBr (H 2 + C**(4p, 1 D) +HBr) (H 2 + C**(4p, 1 S) +HBr) H 2 + C**(5p, 1 D) +HBr H 2 + C**(5p, 1 S) +HBr H 2 + C**(6p, 1 D) +HBr H 2 + C**(6p, 1 S) +HBragust,heima,...Dec09/AFSTODUMYND-190809hrh-101209ak.pxp

19 75207.18/2 1 D->->5p, 1 D H 2 + C +HBr 59329 H 2 + C*( 1 D) +HBr 69521.63 75207.18/2 1 D->->5p, 1 D 5685.55 H 2 + C**( 3 D) +HBr H 2 + C**( 3 P) +HBr (H 2 + C**(4p, 1 D) +HBr) (H 2 + C**(4p, 1 S) +HBr) H 2 + C**(5p, 1 D) +HBr H 2 + C**(5p, 1 S) +HBr H 2 + C**(6p, 1 D) +HBr H 2 + C**(6p, 1 S) +HBragust,heima,...Dec09/AFSTODUMYND-190809hrh-101209ak.pxp

20 77025.63/2 1 D->->6p, 1 D H 2 + C +HBr 59329 H 2 + C*( 1 D) +HBr 69521.63 77025.63/2 1 D->->6p, 1 D 7504 H 2 + C**( 3 D) +HBr H 2 + C**( 3 P) +HBr (H 2 + C**(4p, 1 D) +HBr) (H 2 + C**(4p, 1 S) +HBr) H 2 + C**(5p, 1 D) +HBr H 2 + C**(5p, 1 S) +HBr H 2 + C**(6p, 1 D) +HBr H 2 + C**(6p, 1 S) +HBragust,heima,...Dec09/AFSTODUMYND-190809hrh-101209ak.pxp

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