1. R & D Status of Lost Alpha Measurement - Development of Scintillators M. Nishiura, M. Isobe, N. Kubo, T. Hirouchi,M. Sasao, K. Shinto, M. Okamoto, S. Kitajima, and S.V. Konovalov NIFS, Tohoku Univ. and Kurchatov Institute OUTLINE  Concept and System Candidates  Location of Detection : the geometrical restriction and orbits of escaping alpha particles  Development of Ceramic Scintillation materials  Summary and Future work

2. 2/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Concept and System Candidates Candidates of Measurement Tools Points- measurement : Energy and pitch-angle resolved Faraday-cup detectors, Scintillator probes, Bolometric Imaging (Peterson et al.) Loss imaging: IR camera imaging, Camera imaging of scintillators on the FW Gamma Ray (Kipty et al.)

3. 3/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Sensors (1)selective sensitivity to alpha particles, (2) low sensitivity to other ions, neurons, electrons (3) stable at high temperature (~ 700 K), (4)wide dynamic range and linearity, (5)mechanical endurance under conditions of high temperature and radiation exposure. Signal types and transfer-methods should be considered. Faraday-cup detectors - current (micro A-mA) Scintillator probes - 400 - 600 nm Bolometric Imaging (IR) Loss imaging: IR camera imaging (IR) Camera imaging of scintillators on the FW - 400 - 600 nm Requirements to the System

4. 4/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Location of Detection : the geometrical restriction FW Ceramic Schintillator The CAMERA upper port 11 viewing Camera imaging:The upper port 11 is used for the viewing camera, and the ceramic scintillators are fixed using blanket gaps and slit, or extra shallow pits. Probes : better to be installed on the bottom of the port plug. Probes (FC, Schintillator, Bolometric) Heat Load (kW/m 2 ) #16#17port

5. 5/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Be FW alpha viewing Ceramic Schintillator EXAMPLE A: Ceramic Schintillators are fixed in holes on the top end of FW (Cu backing) of the BM #17 and view from the upper port camera. A Location of Detection : the geometrical restriction A X

6. 6/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Orbit calculation for Detector position A The detector position A, is not good, by two reasons. 1) Drift orbits might not touch the wall surface ? (should be confirmed ). 2) The poloidal angle of the lost position is not the best  A A A

7. 7/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Orbit calculation for Detector position B Detector position B : Moving upward poloidally along the slits on the BM #16, drift orbits cover wider area of returning position. Those might be suitable to observe the MHD loss. There might be possibility to observe alpha losses with probes on the bottom of port plug. However, the coverage of wider area of poloidal angle is needed as the basic understanding.  Extra Holes

8. 8/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Development of Ceramic Scintillation materials Two applications Scintillator probes Camera imaging of scintillators on the FW The required properties of a scintillation plate to be used on ITER are as follows: (1)high sensitivity to alpha particles, (2) low sensitivity to other ions, neurons, electrons, gamma rays, (3) stable emission at high temperature (~ 700 K), (4)Wide dynamic range and liniearity, (5)mechanical endurance under conditions of high temperature and radiation exposure. (6)No-irradiation damage It had been known that the sensitivity of ceramic scintillator diminishes under high temperature, above 100 o C. The characteristics of ceramic sheets in which scintillation materials are blended have been tested.

9. 9/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Comparison of Scintillation materials

10. 10/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Mix scintillation materials, ceramic bond, and H 2 O Dry in room temperature Baking in vacuum at T>150 ℃ Y 3 Al 5 O 12 :Ce ※ ceramic bond Y 3 Al 5 O 12 :Ce Scintillation plates Fabrication of ceramic-like Scintillation plates The reference : ZnS(Ag) which is deposited on the glass plate is tested. LHD lost ion probe uses this type.

11. 11/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Irradiation experiment at 4.5 MV-Dynamitron(FNL) at Tohoku Univ. Bombardment by p, 4 He, at 1- 100 nA Irradiation stage is equipped with –Optical Fiber head to a spectrometer (PM-1) –FC, CCD camera –Heaters, thermo-couples 4.5MV- Dynamitron Scintillator Heater and thermo couple Spectrometor Beam transport line Scinntillator test chamber Scintillator test chamber

12. 12/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Results from 3MeV H +, He + Beam bombardment Experimental results for the ceramic-like scintillators - preheated at 150 ℃ The linearity of the emission intensity to the beam influx is good up to > 4x10 12 ions/(cm 2 s). Typical influx expected at ITER is ranging in 10 12 ~ 10 14 ions/(cm 2 s) But the degradation was observed soon after one minute beam irradiation. Typical video image for Y 3 Al 5 O 12 :Ce with Aron ceramic Beam intensity changed. Synergetic Effect of Temperature and Irradiation

13. 13/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Irradiation damage of YAG:Ce and ZnS:Ag at the room temperature Before beam irradiation, the heat treatment up to 450 ºC had been carried out for two hours. YAG:Ce He + beam current (nA) ◇ 36.50,□37.10, △ 37.05, ◇ 36.65,□34.25, △ 35.6, ◇ 35.25,□35.75 Flux ~1.8x 10 12 ions/(cm 2 s) The substrate temperature keeps constant at 17 ºC during the beam irradiation. ZnS:Ag He + beam current (nA) ◇ 34.25,□36.00, △ 36.50, ◇ 34.00 room temperature YAG:Ce ZnS:Ag Irradiation time (min.) 0 0160 30

14. 14/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Effect of pre-heating treatment on the irradiation degradation. Before beam irradiation, the heat treatment up to 450 ºC had been carried out for two hours. From above equations, the time constant of the degradation can be obtained as  wo =77, and  w =100. After a year operation, t=10 7 /60 min, the intensity degradation with baking becomes smaller than that without baking. It is found that the emission intensity becomes 0.33 of the original. YAG:Ce withAaron ceramic

15. 15/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Dependence of emission for YAG:Ce and ZnS:Ag on temperature YAG:Ce 450 ºC, two hours baking before experiments ZnS:Ag 400 ºC, two hours baking before experiments He + beam current (nA) ◇38.00, □ 36.50,△36.00 After the irradiation, the degradation of the fluorescent intensity is observed. YAG:Ce ZnS:Ag Present data From Z. Lin et al. PPPL TM392

16. 16/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Summary and Future work Studies of ITER integration for several systems are started. Ceramic-like schintillation-material can be fixed in shallow pits on the FW, and viewed from the upper port camera of #11. Probes for energy and angle-resolved measurement, Faraday-cup detectors, scintillator probes, Bolometric Imaging detectors can be installed in the bottom of diagnostic ports. Full-gyro orbit calculations including realistic detector designs and detailed 3D FW shapes, are needed, and now under preparation. The ceramic schintillators newly developed were tested with 1-3 MeV alpha beam and the linearity of the emission intensity to the beam influx is good up to > 4x10 12 ions/(cm 2 s). Typical influx expected at FW of ITER is ranging in 10 12 ~ 10 14 ions/(cm 2 s)

17. 17/14 10th ITPA diagnostics meeting, Moscow 10-14/04/06M. Sasao Summary and Future work The ceramic schintillators newly developed were tested with 1-3 MeV alpha beam. The test under high temperature shows that the efficiency of some ceramic schintillators does not change on temperature upto 300 ºC, but changes by dose accumulation. Irradiation effect is large for ZnS:Ag, but less for a ceramic-like schintillators of YAG:Ce, and it becomes stronger by preheating treatment. -> One year operation of ITER corresponds to continuous bombardment of flux of 140 min.:1.8x 10 12 ions/cm 2 /s, total fluence:9x10 17 ions/(cm 2 ) ． Our present experimental test showed that degradation of emission efficiency of a ceramic- like schintillators of YAG:Ce is less than 33%. A experiment to test improvement by heating recovering treatment is planned.