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Superconductivity and non-Fermi-liquid behavior of Ce 2 PdIn 8 V. H. Tran et al., PHYSICAL REVIEW B 83, 064504 (2011) Kitaoka Lab. M1 Ryuji Michizoe.

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Presentation on theme: "Superconductivity and non-Fermi-liquid behavior of Ce 2 PdIn 8 V. H. Tran et al., PHYSICAL REVIEW B 83, 064504 (2011) Kitaoka Lab. M1 Ryuji Michizoe."— Presentation transcript:

1 Superconductivity and non-Fermi-liquid behavior of Ce 2 PdIn 8 V. H. Tran et al., PHYSICAL REVIEW B 83, 064504 (2011) Kitaoka Lab. M1 Ryuji Michizoe

2 Contents ・ Introduction - History of Superconductivity - Heavy fermion system ・ Results ・ Summary

3 under high pressure 0 50 100 150 200 SmO 0.9 F 0.11 FeAs LaO 0.89 F 0.11 FeAs LaOFeP Hg-Ba-Ca-Cu-O () Tl-Ba-Ca-Cu-O Bi-Sr-Ca-Cu-O Y-Ba-Cu-O MgB 2 NbGe NbN NbC Nb Pb high-T c cuprate metal iron-based system SC transition temperature-T c (K) 1900192019401960198020002020 Year Hg La-Ba-Cu-O Discovery of superconducting phenomenon 1911 1986 High-T c cuprate superconductor 2006 Iron-based high-T c superconductor 77 163 History of Superconductivity(SC) 1979 Heavy fermion superconductor CeCu 2 Si 2 heavy fermion system PuCoGa 5

4 UPt 3 UPd 2 Al 3 CeCu 2 Si 2 CePd 2 Si 2 CeRh 2 Si 2 CeIn 3 CeRhIn 5 PrOs 4 Sb 12 PuCoGa 5 etc f electrons Heavy fermion compounds n(r)n(r) r 4f4f 5p5p 5d5d 6s6s

5 ++ ff + f ++ ff + f Heavy fermion state Normal metal +++ +++ Heavy fermion state c-f hybridization conduction electron

6 J cf Polarization The interplay between two 4f electrons mediated by conduction electrons Heavy fermion system Heavy fermion system RKKY interaction Conduction electron 4f electron Magnetic Order

7 Heavy fermion system Heavy fermion system 4f and conduction electrons form a spin-singlet state Kondo effect J cf Conduction electron 4f electron Fermi Liquid

8 T K ∝ W exp(-1/J cf D(ε F )) T RKKY ∝ D(ε F ) J cf 2 Phase Diagram of HF system AFM : antiferromagnetism HF : heavy fermion state QCP : quantum critical point

9 Kondo effect 4f electron Kondo effect Conduction electron

10 P dependence of T max Above T max Incoherent Kondo scattering Below T max Coherent Kondo scattering

11 T max shifts to high T P dependence of T max T max ∝ T K

12 Resistivity of Ce 2 PdIn 8 P decreases T c 1 bar T c ~ 0.7 K

13 The P dependence of T C P suppresses SC P ~ 21 kbar SC disappears

14 Non-Fermi-liquid behavior Fermi-liquid ρ(T ) = ρ 0 + AT 2 ρ(T ) = ρ 0 + AT n (n < 2) n = 1 : 2D antiferromagnetic spin fluctuation n = 1.5 : 3D antiferromagnetic spin fluctuation n = 2 : Fermi-liquid Non-Fermi-liquid

15 P dependent values of n, A, ρ 0 ρ(T ) = ρ 0 + AT n n = 1 : 2D antiferromagnetic spin fluctuation n = 1.5 : 3D antiferromagnetic spin fluctuation n = 2 : Fermi-liquid A ∝ T K -2

16 P dependent values of n, A, ρ 0 ρ(T ) = ρ 0 + AT n n = 1 : 2D antiferromagnetic spin fluctuation n = 1.5 : 3D antiferromagnetic spin fluctuation n = 2 : Fermi-liquid AF spin fluctuation is supressed by increasing P V. A. Sidorov et al., PRL 89.157004 (2002)

17 SC may be associated with AF spin fluctuation The relationship between SC and AF spin fluctuation

18 non-Fermi-liquid Fermi-liquid T FL : Fermi-liquid temperature Field dependence of resistivity Below H c2 = 2.5 T ρ(T ) ∝ AT Above H c2 = 2.5 T ρ(T ) ∝ AT 2 n = 1 : 2D antiferromagnetic spin fluctuation n = 1.5 : 3D antiferromagnetic spin fluctuation n = 2 : Fermi-liquid

19 T FL increases with rising field Fermi-liquid is recovered at strong magnetic fields Field dependence of resistivity

20 Field dependent values of n, A, ρ 0 near H c2 n : jump to n = 2 A : maximum ρ 0 : minimum AF spin fluctuations associated with a QCP Fermi-liquid ρ(T ) = ρ 0 + AT n H c2 n = 1 : 2D antiferromagnetic spin fluctuation n = 1.5 : 3D antiferromagnetic spin fluctuation n = 2 : Fermi-liquid

21 Summary H c2 n = 1 : 2D antiferromagnetic spin fluctuation n = 1.5 : 3D antiferromagnetic spin fluctuation n = 2 : Fermi-liquid SC in Ce 2 PdIn 8 may be mediated by the AF spin fluctuations

22 END

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24 H. Fukazawa et al., PHYSICAL REVIEW B 86, 094508 (2012) Ce 2 PdIn 8

25 Heavy fermion system Heavy fermion system (RKKY:Rudermann-Kittel-Kasuya- Yoshida) Magnetic OrderFermi Liquid Conduction electron 4f electron RKKY interaction The interplay between two 4f electrons mediated by conduction electrons 4f electron Kondo effect 4f and conduction electrons form a spin- singlet state. Conduction electron heavy fermion system : 重い電子系

26 field dependence of the resistivity at 1 bar μ 0 H < 3 T T max ⇒ no change μ 0 H > 3 T T max ⇒ toward lower temperature suppress spin fluctuation

27 Kondo interaction strength(C K ) C K decreases with P C k : Kondo interaction strength

28 C K ~ J 3 N(E F ) 2 J : hybridization N(E F ) : density of states at Fermi level P enhances J N(E F ) strongly diminishes C K decreases P dependence of C K C K decreases with P but

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