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Identification of Active Edge Sites for Electrochemical H 2 Evolution from MoS 2 Nanocatalysts by Thomas F. Jaramillo, Kristina P. Jørgensen, Jacob Bonde,

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Presentation on theme: "Identification of Active Edge Sites for Electrochemical H 2 Evolution from MoS 2 Nanocatalysts by Thomas F. Jaramillo, Kristina P. Jørgensen, Jacob Bonde,"— Presentation transcript:

1 Identification of Active Edge Sites for Electrochemical H 2 Evolution from MoS 2 Nanocatalysts by Thomas F. Jaramillo, Kristina P. Jørgensen, Jacob Bonde, Jane H. Nielsen, Sebastian Horch, and Ib Chorkendorff Science Volume 317(5834):100-102 July 6, 2007 Published by AAAS

2 Fig. 1. A series of STM images of MoS2 nanoparticles on Au(111). Thomas F. Jaramillo et al. Science 2007;317:100-102 Published by AAAS

3 Fig. 2. Polarization curves and Tafel plots in a cathodic potential window for the five different MoS2 samples as well as a blank sample. Thomas F. Jaramillo et al. Science 2007;317:100-102 Published by AAAS

4 Fig. 3. Exchange current density versus (A) MoS2 area coverage and (B) MoS2 edge length. Thomas F. Jaramillo et al. Science 2007;317:100-102 Published by AAAS

5 Fig. 4. Volcano plot of the exchange current density as a function of the DFT-calculated Gibbs free energy of adsorbed atomic hydrogen for nanoparticulate MoS2 and the pure metals (23). Thomas F. Jaramillo et al. Science 2007;317:100-102 Published by AAAS


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