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Kondo effect in a quantum dot without spin Hyun-Woo Lee (Postech) & Sejoong Kim (Postech MIT) References: H.-W. Lee & S. Kim, cond-mat/0610496 P. Silvestrov & Y. Imry, cond-mat/0609355 V. Kashcheyevs, A. Schiller, A. Aharony, & O. Entin-Wohlman, cond-mat/0610194
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Kondo effect Temperature dependence of resistance Resistance minimum
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Kondo effect (continued) [J. Kondo, Prog. Theor. Phys. ’64] Scattering by magnetic impurities Before After s - d model
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Scattering amplitude for a channel of where N : number of d-electrons, N(0) : density of state at E F D : width of conduction electron distribution around E F This lnT dependence combined with the phonon contribution ( T 5 dependence) makes a resistance minimum in R(T). LogT dependence in R(T) J k,q = J where –D < k, q < D = 0 otherwise (*) 엄종화
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Kondo effect (continued) High T vs. low T Kondo singlet Cf. Asymptotic freedom
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T K ~ T 일 때, Hamann expression (Phys. Rev. 1967) For T K > T, take (-) in the equation T K < T, take (+) in the equation T K << T 일 때, When T << T K, ~ 0 - cT 2 : unitary limit Kondo effect (*) 엄종화
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Kondo effect in AuFe(26ppm) wire Hamann expression (Phys. Rev. 1967) From fitting the Hamann expression to (T), we obtain S = 0.12, T K = 0.99 K. Concentration of AuFe is estimated by the slope of => 26 ppm in the above figure Slope of Kondo resistivity = 0.11 n cm / (ppm decade K) (*) 엄종화
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Kondo effect in quantum dot
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Quantum dot (QD) “Metallic” limit ~ e 2 /2C >> kT n VgVg
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Transport through a QD Orthodox theory of Coulomb blockade Transport due to charge fluctuations Transport due to charge fluctuations
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Quantum confinement Single particle energy quantization E >> kT
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Even-odd effect Spin singlet (S=0) vs doublet (S=1/2) QD with odd n = magnetic impurity ??? n VgVg 1 2 3 0 1/2 0 S=1/2
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Kondo effect in QD ? Hamiltonian Spin flip via second order processes c.f. n VgVg Before After
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Kondo effect in QD w/ odd n Theories T. K. Ng and P. A. Lee T. K. Ng and P. A. Lee Phys. Rev. Lett. 61, 1768 (1988)Phys. Rev. Lett. 61, 1768 (1988) L. I. Glazman and M. E. Raikh L. I. Glazman and M. E. Raikh JETP Lett. 47, 452 (1988)JETP Lett. 47, 452 (1988) Experiments D. Goldhaber-Gordon, H. Shtrikman, D. Mahalu, D. Abush-Magder, U. Meirav, and M. A. Kaster D. Goldhaber-Gordon, H. Shtrikman, D. Mahalu, D. Abush-Magder, U. Meirav, and M. A. Kaster Nature 391, 156 (1998); Phys. Rev. Lett. 81, 5225 (1998)Nature 391, 156 (1998); Phys. Rev. Lett. 81, 5225 (1998) S. M. Cronenwett, T. H. Oostercamp, and L. P. Kouwenhoven S. M. Cronenwett, T. H. Oostercamp, and L. P. Kouwenhoven Science 281, 540 (1998)Science 281, 540 (1998) Kondo suppression of Kondo suppression of R
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Unitary limit of the Kondo effect in SET [W. G. van der Wiel et al., Science ’00] G at V gl = -413mV shows logarithmic T dependence (inset), and saturates below 90mK (unitary limit) This experiment shows a unitary limit = 2 e 2 / h ( R = L 의 경우 ) V gl was fixed at -413mV. V SD was biased between S and D. Kondo resonance peak G(T)G(T) 온도대역 : 15 mK – 800 mK FWHM (*) 엄종화
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Kondo temperature: T K ; Costi et al., J. Phys.: Condense. Matter 6, 2519 (1994) In Anderson model, An empirical function ; Goldhaber-Gordon et al., PRL 81, 5225 (1998) T K in Log scale : universal functional form of T / T K s is a fit parameter, but is almost constant ~0.2 in the Kondo regime. (*) 엄종화
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Kondo effect in QD w/o spin?
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Beyond orthodox theory Anomalous transmission phase Yacoby et al., PRL 74, 4047 (1995); Schuster et al., Nature 385, 417 (1997); Avinun-Khalish et al., Nature 436, 529 (2005) Yacoby et al., PRL 74, 4047 (1995); Schuster et al., Nature 385, 417 (1997); Avinun-Khalish et al., Nature 436, 529 (2005) Bruder et al., PRL 76, 114 (1995); Lee, PRL 82, 2358 (1999); Silvestrov et al., PRL 85, 2565 (2000) Bruder et al., PRL 76, 114 (1995); Lee, PRL 82, 2358 (1999); Silvestrov et al., PRL 85, 2565 (2000) Population switching Silvestrov et al., PRL 85, 2565 (2000); Konig et al., PRB 71, R201308 (2005); Sindel et al., PRB 72, 125316 (2005) Silvestrov et al., PRL 85, 2565 (2000); Konig et al., PRB 71, R201308 (2005); Sindel et al., PRB 72, 125316 (2005) Correlation-induced resonace Meden et al., PRL 96, 146801 (2006); PRB 73, 235337 (2006) Meden et al., PRL 96, 146801 (2006); PRB 73, 235337 (2006)
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Two level QD QD w/ two single-particle level Source & Drain Tunneling “Spin” ? t1Lt1L t1Rt1R t2Lt2L t1Rt1R tt
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Pseudospin for 1 = 2 (= ) Unitary transformations Pseudospin Pseudospin up Pseudospin down
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Schrieffer-Wolf transformation: QD system (Anderson model) s - d model Fock space decomposition Full Hamiltonian Projection to n =1 Fock space 012
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Effective Hamiltonian H s-d Total Hamiltonian Anisotropic antiferro-exchange Anisotropic antiferro-exchange U(1) instead of SU(2)U(1) instead of SU(2) Pseudomagnetic field B z eff Pseudomagnetic field B z eff (*) For = (*) For = SU(2): J z =J + =J -SU(2): J z =J + =J - B z eff =0B z eff =0
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Pseudomagnetic field B z eff Expectation value For > For > Population switching from level to level with decreasing Population switching from level to level with decreasing 0-U/2 =+U/2 012 hzhz
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Population switching (PS) [Silvestrov & Imry, PRL’00] Energy renormalization eff = bare + (hopping) eff = bare + (hopping) : gate voltage dependent : gate voltage dependent Charge 1 0 U U Charge 1 2 0-U/2 =+U/2 012
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Poor man’s scaling [1] Fock space decomposition [2] Full Hamiltonian [3] Projection to “g” sector of Fock space New Hamiltonian w/ reduced D New Hamiltonian w/ reduced D [4] Back to [1] D DD DD
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Scaling equations Exchange J ’s Scaling invariant Scaling invariant Integration: Characteristic energy scale (Kondo temperature) Integration: Characteristic energy scale (Kondo temperature) Pseudomagnetic field B z eff Integration: Integration:
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Anisotropic s - d model Approximation Anisotropic s - d model Exact solution (via Bethe ansatz) available !!! Exact solution (via Bethe ansatz) available !!! Tsvelick & Wiegmann, Adv. Phys. 32, 453 (1983)Tsvelick & Wiegmann, Adv. Phys. 32, 453 (1983)
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Conductance at T=0 and scattering states Friedel sum rule Landauer-Buttiker formula
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Anisotropic s - d model [Tsvelick and Wiegmann, Adv. Phys. (1983)] S z =( n - n )/2 vs. h z G vs.
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Cf. Conventional spin Kondo Conventional spin Kondo Kondo w/o spin Correlation-induced resonance Correlation-induced resonance [Meden & Marquardt, PRL 96, 146801 (2006)] 0-U/2 =+U/2 012
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w/o degeneracy 1 - 2 0 Same Unitary transformation Additional pseudomagnetic field h Parallel to z Parallel to z Shift of CIRsShift of CIRs Perpendicular to z Perpendicular to z Asymmetry in CIRs (Fano-like)Asymmetry in CIRs (Fano-like)
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Summary Kondo effect in QD w/o spin Distinct conductance pattern (cf. spin Kondo in QD) Distinct conductance pattern (cf. spin Kondo in QD) Future directions w/o degeneracy w/o degeneracy Temperature dependence Temperature dependence Pseudospin & real spin Pseudospin & real spin Real Spin [SU(2)]Real Spin [SU(2)] Pseudospin [Not SU(2) invariant]Pseudospin [Not SU(2) invariant] Connection w/ anomalous transmission phase problem ?Connection w/ anomalous transmission phase problem ?
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